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A Topographic View of Supercooled Liquids and Glass Formation
Abstract
Various static and dynamic phenomena displayed by glass-forming liquids, particularly those near the so-called "fragile" limit, emerge as manifestations of the multidimensional complex topography of the collective potential energy function. These include non-Arrhenius viscosity and relaxation times, bifurcation between the α- and β-relaxation processes, and a breakdown of the Stokes-Einstein relation for self-diffusion. This multidimensional viewpoint also produces an extension of the venerable Lindemann melting criterion and provides a critical evaluation of the popular "ideal glass state" concept.
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Cited by
Characteristics and Significance of the Amorphous State in Pharmaceutical Systems
Hancock, B. C., & Zografi, G. (1997) · Journal of Pharmaceutical Sciences · doi:10.1021/js9601896 · Cited by 1,922
Atomic-level structure and structure–property relationship in metallic glasses
Cheng, Y. Q., & Ma, E. (2011) · Progress in Materials Science · doi:10.1016/j.pmatsci.2010.12.002 · Cited by 1,771
A phase diagram for jammed matter
Song, C., Wang, P., & Makse, H. A. (2008) · Nature · doi:10.1038/nature06981 · Cited by 964
Atomic Level Structure in Multicomponent Bulk Metallic Glass
Cheng, Y. Q., Ma, E., & Sheng, H. W. (2009) · Physical Review Letters · doi:10.1103/physrevlett.102.245501 · Cited by 916
Complex plasmas: An interdisciplinary research field
Morfill, G. E., & Ivlev, A. V. (2009) · Reviews of Modern Physics · doi:10.1103/revmodphys.81.1353 · Cited by 803
Metadata
- Authors
- Stillinger, F. H.
- Venue
- Science
- Published
- 1995-03-31
- Volume
- 267
- Issue
- 5206
- Pages
- 1935-1939
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1997676547
- Cited by
- 1,467
- References
- 0
- FWCI
- 31.43
- Type
- journal article
- Language
- en
- Open access
- closed
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
