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A synthetic Mn 4 Ca-cluster mimicking the oxygen-evolving center of photosynthesis
Open accessAbstract
Mimicking the oxygen evolution center: Making a synthetic analog of plant photosynthesis is a key goal for exploiting solar energy and replacing fossil fuels. Zhang et al. synthesized a manganese-calcium cluster that looks and acts like the oxygen evolution center in photosystem II (see the Perspective by Sun). The mimic structurally resembles the biological complex, with the notable exception of bridging protein ligands and water-binding sites on a dangling Mn atom. Functionally, however, the cluster's metal center readily undergoes four redox transitions, which contribute to splitting water into oxygen. This and other synthetic mimics will pave the way for developing more efficient catalysts for artificial photosynthesis. Science , this issue p. 690 ; see also p. 635
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Cites
Photosynthetic energy conversion: natural and artificial
Barber, J. (2009) · Chem. Soc. Rev. · doi:10.1039/b802262n · Cited by 1,843
Cited by
Zhao, Y., Waterhouse, G. I. N., Chen, G., Xiong, X., Wu, L.-Z., Tung, C.-H., & Zhang, T. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00607e · Cited by 435
Challenges and opportunities for hydrogen production from microalgae
Oey, M., Sawyer, A. L., Ross, I. L., & Hankamer, B. (2016) · Plant Biotechnology Journal · doi:10.1111/pbi.12516 · Cited by 180
Bioinspired and Bioderived Aqueous Electrocatalysis
Barrio, J., Pedersen, A., Favero, S., Luo, H., Wang, M., Sarma, S. C., Feng, J., Ngoc, L. T. T., Kellner, S., Li, A. Y., et al. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00429 · Cited by 80
Metadata
- Authors
- Zhang, C., Chen, C., Dong, H., Shen, J.-R., Dau, H., & Zhao, J.
- Venue
- Science
- Published
- 2015-05-08
- Volume
- 348
- Issue
- 6235
- Pages
- 690-693
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1519008653
- Cited by
- 496
- References
- 1
- FWCI
- 25.76
- Type
- journal article
- Language
- en
- Open access
- bronze
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