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Wafer-scale synthesis of monolayer two-dimensional porphyrin polymers for hybrid superlattices
Abstract
Single-layer porphyrin polymerization: Two-dimensional polymers can be made as monolayer sheets through controlled synthesis at an interface. However, it is often difficult to create intact sheets over large areas that can be transferred onto substrates. Zhong et al. polymerized derivatized porphyrin molecules during laminar flow at a sharp pentane-water interface to form sheets that are 5 centimeters in diameter (see the Perspective by MacLean and Rosei). The authors used electron microscopy and spectroscopy to confirm that they had produced intact monolayers. These films were then transferred onto monolayer sheets of molybdenum disulfide to form superlattices for use as capacitors. Science , this issue p. 1379 ; see also p. 1308
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Cited by
New synthetic strategies toward covalent organic frameworks
Li, Y., Chen, W., Xing, G., Jiang, D., & Chen, L. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00199f · Cited by 658
Interfacial Polymerization: From Chemistry to Functional Materials
Zhang, F., Fan, J., & Wang, S. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201916473 · Cited by 478
2D Materials in Flexible Electronics: Recent Advances and Future Prospectives
Katiyar, A. K., Hoang, A. T., Xu, D., Hong, J., Kim, B. J., Ji, S., & Ahn, J.-H. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.3c00302 · Cited by 363
Yan, Y., Li, C., Wu, Y., Gao, J., & Zhang, Q. (2020) · Journal of Materials Chemistry A · doi:10.1039/d0ta03749d · Cited by 260
Metadata
- Authors
- Zhong, Y., Cheng, B., Park, C., Ray, A., Brown, S., Mujid, F., Lee, J.-U., Zhou, H., Suh, J., Lee, K.-H., Mannix, A. J., Kang, K., Sibener, S. J., Muller, D. A., & Park, J.
- Venue
- Science
- Published
- 2019-12-13
- Volume
- 366
- Issue
- 6471
- Pages
- 1379-1384
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2983797573
- Cited by
- 269
- References
- 0
- FWCI
- 12.42
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhong, Y., Cheng, B., Park, C., Ray, A., Brown, S., Mujid, F., Lee, J.-U., Zhou, H., Suh, J., Lee, K.-H., Mannix, A. J., Kang, K., Sibener, S. J., Muller, D. A., & Park, J. (2019). Wafer-scale synthesis of monolayer two-dimensional porphyrin polymers for hybrid superlattices. Science. https://doi.org/10.1126/science.aax9385
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