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Redox reactions of small organic molecules using ball milling and piezoelectric materials
Open accessAbstract
Redox catalysis in a ball mill: Mixing solid reactants in a ball mill is a promising means of avoiding the copious solvent waste associated with most chemical syntheses. Kubota et al. now report that adding a piezoelectric catalyst to the mix can promote bond formation through apparent electron transfer cycles (see the Perspective by Xia and Wang). Specifically, barium titanate activates aryl diazonium salts toward borylation and coupling with heterocycles in a manner reminiscent of solutionphase photoredox catalysis. The reactions are insensitive to air and were demonstrated up to gram scale. Science , this issue p. 1500 ; see also p. 1451
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Prier, C. K., Rankic, D. A., & MacMillan, D. W. C. (2013) · Chemical Reviews · doi:10.1021/cr300503r · Cited by 9,590
Piezoelectric Nanogenerators Based on Zinc Oxide Nanowire Arrays
Wang, Z. L., & Song, J. (2006) · Science · doi:10.1126/science.1124005 · Cited by 7,922
Cited by
Tu, S., Guo, Y., Zhang, Y., Hu, C., Zhang, T., Ma, T., & Huang, H. (2020) · Advanced Functional Materials · doi:10.1002/adfm.202005158 · Cited by 986
Recent Development of Aryl Diazonium Chemistry for the Derivatization of Aromatic Compounds
Mo, F., Qiu, D., Zhang, L., & Wang, J. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c01030 · Cited by 361
Mechanochemistry: New Tools to Navigate the Uncharted Territory of “Impossible” Reactions
Cuccu, F., De Luca, L., Delogu, F., Colacino, E., Solin, N., Mocci, R., & Porcheddu, A. (2022) · ChemSusChem · doi:10.1002/cssc.202200362 · Cited by 339
Ferro-catalysis Bioelectronics: Progress and Prospects
Tang, X., Liu, Y., Li, L., Song, Y., Dai, Y., Yang, Y., Yuan, G., & Wang, Y. (2024) · Nano Energy · doi:10.1016/j.nanoen.2023.109059 · Cited by 8
Metadata
- Authors
- Kubota, K., Pang, Y., Miura, A., & Ito, H.
- Venue
- Science
- Published
- 2019-12-20
- Volume
- 366
- Issue
- 6472
- Pages
- 1500-1504
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2995918333
- Cited by
- 603
- References
- 2
- FWCI
- 19.32
- Type
- journal article
- Language
- en
- Open access
- green
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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