The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Maximizing noble metal utilization in solid catalysts by control of nanoparticle location
Open accessAbstract
Maximizing the utilization of noble metals is crucial for applications such as catalysis. We found that the minimum loading of platinum for optimal performance in the hydroconversion of n -alkanes for industrially relevant bifunctional catalysts could be reduced by a factor of 10 or more through the rational arranging of functional sites at the nanoscale. Intentionally depositing traces of platinum nanoparticles on the alumina binder or the outer surface of zeolite crystals, instead of inside the zeolite crystals, enhanced isomer selectivity without compromising activity. Separation between platinum and zeolite acid sites preserved the metal and acid functions by limiting micropore blockage by metal clusters and enhancing access to metal sites. Reduced platinum nanoparticles were more active than platinum single atoms strongly bonded to the alumina binder.
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Cites
Ultralow-loading platinum-cobalt fuel cell catalysts derived from imidazolate frameworks
Chong, L., Wen, J., Kubal, J., Sen, F. G., Zou, J., Greeley, J., Chan, M., Barkholtz, H., Ding, W., & Liu, D.-J. (2018) · Science · doi:10.1126/science.aau0630 · Cited by 1,100
Polyethylene upcycling to long-chain alkylaromatics by tandem hydrogenolysis/aromatization
Zhang, F., Zeng, M., Yappert, R. D., Sun, J., Lee, Y.-H., LaPointe, A. M., Peters, B., Abu-Omar, M. M., & Scott, S. L. (2020) · Science · doi:10.1126/science.abc5441 · Cited by 882
Cited by
Dong, Z., Chen, W., Xu, K., Liu, Y., Wu, J., & Zhang, F. (2022) · ACS Catalysis · doi:10.1021/acscatal.2c04915 · Cited by 269
Wang, C., Guo, W., Chen, T., Lu, W., Song, Z., Yan, C., Feng, Y., Gao, F., Zhang, X., Rao, Y., et al. (2024) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2024.215899 · Cited by 184
Self-citationCao, Y., Yu, X., Wang, T., Li, J., Li, N., Ge, A., Ying, J., & Yu, T. (2024) · Chemistry - An Asian Journal · doi:10.1002/asia.202400342 · Cited by 9
Metadata
- Authors
- Cheng, K., Smulders, L. C. J., van der Wal, L. I., Oenema, J., Meeldijk, J. D., Visser, N. L., Sunley, G., Roberts, T., Xu, Z., Doskocil, E., Yoshida, H., Zheng, Y., Zečević, J., de Jongh, P. E., & de Jong, K. P.
- Venue
- Science
- Published
- 2022-07-08
- Volume
- 377
- Issue
- 6602
- Pages
- 204-208
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W4284694916
- Cited by
- 242
- References
- 2
- FWCI
- 14.54
- Type
- journal article
- Language
- en
- Open access
- green
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- Cheng, K., Smulders, L. C. J., van der Wal, L. I., Oenema, J., Meeldijk, J. D., Visser, N. L., Sunley, G., Roberts, T., Xu, Z., Doskocil, E., Yoshida, H., Zheng, Y., Zečević, J., de Jongh, P. E., & de Jong, K. P. (2022). Maximizing noble metal utilization in solid catalysts by control of nanoparticle location. Science. https://doi.org/10.1126/science.abn8289
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