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Structural destabilization induced by lithium intercalation in MoS2 and related compounds
Open accessAbstract
2H-MoS 2 is a semiconductor with a hexagonal layered structure. Each Mo atom is prismatically coordinated by six S atoms. Our in situ X-ray diffraction results indicate that, upon intercalation, the MoS 2 host lattice undergoes a first order phase transition in which the Mo coordination changes from trigonal prismatic to octahedral (1T structure). The driving mechanism for this structural change is discussed in terms of a charge transfer from the lithium to the host and in terms of the respective energy-band diagrams for 2H and 1T polytypes. Intercalation-induced reversals in the relative stability of trigonal–prismatic and octahedral phases may also be expected in other semiconducting hosts.
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Cited by
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Photoluminescence from Chemically Exfoliated MoS 2
Eda, G., Yamaguchi, H., Voiry, D., Fujita, T., Chen, M., & Chhowalla, M. (2011) · Nano Letters · doi:10.1021/nl201874w · Cited by 3,896
Enhanced Hydrogen Evolution Catalysis from Chemically Exfoliated Metallic MoS 2 Nanosheets
Lukowski, M. A., Daniel, A. S., Meng, F., Forticaux, A., Li, L., & Jin, S. (2013) · Journal of the American Chemical Society · doi:10.1021/ja404523s · Cited by 3,341
Enhanced catalytic activity in strained chemically exfoliated WS2 nanosheets for hydrogen evolution
Voiry, D., Yamaguchi, H., Li, J., Silva, R., Alves, D. C. B., Fujita, T., Chen, M., Asefa, T., Shenoy, V. B., Eda, G., et al. (2013) · Nature Materials · doi:10.1038/nmat3700 · Cited by 2,641
Lv, R., Robinson, J. A., Schaak, R. E., Sun, D., Sun, Y., Mallouk, T. E., & Terrones, M. (2015) · Accounts of Chemical Research · doi:10.1021/ar5002846 · Cited by 1,380
Metadata
- Authors
- Py, M. A., & Haering, R. R.
- Venue
- Canadian Journal of Physics
- Publisher
- Canadian Science Publishing
- Published
- 1983-01-01
- Volume
- 61
- Issue
- 1
- Pages
- 76-84
- ISSN
- 0008-4204 (ISSN-L)
- 1208-6045
- OpenAlex
- W2052434745
- Cited by
- 650
- References
- 0
- FWCI
- 5.39
- Type
- journal article
- Language
- en
- Open access
- green
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- Py, M. A., & Haering, R. R. (1983). Structural destabilization induced by lithium intercalation in MoS2 and related compounds. Canadian Journal of Physics. https://doi.org/10.1139/p83-013
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