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Carbon Metal Fluoride Nanocomposites
Open accessAbstract
The structure and electrochemistry of -based carbon metal fluoride nanocomposites (CMFNCs) was investigated in detail from 4.5 to 1.5 V, revealing a reversible metal fluoride conversion process. These are the first reported examples of a high-capacity reversible conversion process for positive electrodes. A reversible specific capacity of approximately 600 mAh/g of CMFNCs was realized at 70°C. Approximately one-third of the capacity evolved in a reaction between 3.5 and 2.8 V related to the cathodic reduction reaction of to The remainder of the specific capacity occurred in a two-phase conversion reaction at 2 V resulting in the formation of a finer Fe:LiF nanocomposite. Upon oxidation, selective area electron diffraction characterization revealed the reformation of a metal fluoride. Evidence presented suggested that the metal fluoride is related to in structure. A pseudocapacitive reaction is proposed as a possible mechanism for the subsequent oxidation reaction. Preliminary results of and CMFNCs were used in the discussion of the electrochemical properties of the reconverted metal fluoride. © 2003 The Electrochemical Society. All rights reserved.
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Cited by
Electrode Degradation in Lithium-Ion Batteries
Pender, J. P., Jha, G., Youn, D. H., Ziegler, J. M., Andoni, I., Choi, E. J., Heller, A., Dunn, B. S., Weiss, P. S., Penner, R. M., et al. (2020) · ACS Nano · doi:10.1021/acsnano.9b04365 · Cited by 873
Metadata
- Authors
- Badway, F., Cosandey, F., Pereira, N., & Amatucci, G. G.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2003
- Volume
- 150
- Issue
- 10
- Pages
- A1318
- ISSN
- 0013-4651 (ISSN-L)
- OpenAlex
- W2099895320
- Cited by
- 443
- References
- 0
- FWCI
- 8.38
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Badway, F., Cosandey, F., Pereira, N., & Amatucci, G. G. (2003). Carbon Metal Fluoride Nanocomposites. Journal of The Electrochemical Society. https://doi.org/10.1149/1.1602454
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