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Li Conductivity in Li[sub x]MPO[sub 4] (M = Mn, Fe, Co, Ni) Olivine Materials
Abstract
Materials with the olivine Li x MPO 4 structure form an important class of rechargeable battery cathodes. Using first-principles methods, activation barriers to Li ion motion are calculated and an estimate for Li diffusion constants, in the absence of electrical conductivity constraints, is made. Materials with M = Mn , Fe, Co, Ni are considered. Li diffuses through one-dimensional channels with high energy barriers to cross between the channels. Without electrical conductivity limitations the intrinsic Li diffusivity is high. © 2003 The Electrochemical Society. All rights reserved.
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Cited by
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Pender, J. P., Jha, G., Youn, D. H., Ziegler, J. M., Andoni, I., Choi, E. J., Heller, A., Dunn, B. S., Weiss, P. S., Penner, R. M., et al. (2020) · ACS Nano · doi:10.1021/acsnano.9b04365 · Cited by 873
Materials Design Rules for Multivalent Ion Mobility in Intercalation Structures
Rong, Z., Malik, R., Canepa, P., Sai Gautam, G., Liu, M., Jain, A., Persson, K., & Ceder, G. (2015) · Chemistry of Materials · doi:10.1021/acs.chemmater.5b02342 · Cited by 561
Self-citationFisher, C. A. J., Hart Prieto, V. M., & Islam, M. S. (2008) · Chemistry of Materials · doi:10.1021/cm801262x · Cited by 549
Recent advances in the research of polyanion-type cathode materials for Li-ion batteries
Gong, Z., & Yang, Y. (2011) · Energy & Environmental Science · doi:10.1039/c0ee00713g · Cited by 549
Takamoto, S., Shinagawa, C., Motoki, D., Nakago, K., Li, W., Kurata, I., Watanabe, T., Yayama, Y., Iriguchi, H., Asano, Y., et al. (2022) · Nature Communications · doi:10.1038/s41467-022-30687-9 · Cited by 446
Metadata
- Authors
- Morgan, D., Van der Ven, A., & Ceder, G.
- Venue
- Electrochemical and Solid-State Letters
- Publisher
- The Electrochemical Society
- Published
- 2004
- Volume
- 7
- Issue
- 2
- Pages
- A30
- ISSN
- 1099-0062 (ISSN-L)
- OpenAlex
- W2260433152
- Cited by
- 1,124
- References
- 0
- FWCI
- 22.23
- Type
- journal article
- Language
- en
- Open access
- closed
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- Morgan, D., Van der Ven, A., & Ceder, G. (2004). Li Conductivity in Li[sub x]MPO[sub 4] (M = Mn, Fe, Co, Ni) Olivine Materials. Electrochemical and Solid-State Letters. https://doi.org/10.1149/1.1633511
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