Cited by 309Fuel Cells and Related MaterialsElectrocatalysts for Energy ConversionAdvancements in Solid Oxide Fuel Cells

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Effects of Microstructure of Carbon Support in the Catalyst Layer on the Performance of Polymer‐Electrolyte Fuel Cells

Uchida, Makoto, Fukuoka, Yuko, Sugawara, Yasushi, Eda, Nobuo, Ohta, Akira·1996·Journal of The Electrochemical Society

DOI 10.1149/1.1836988

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Abstract

Effects of microstructure of carbon supports for platinum catalyst and of perfluorosulfonate‐ionomer (PFSI) distribution in the microstructure of the catalyst layer on the consequent performance of polymer‐electrolyte fuel cells, prepared by a new method based on the process of PFSI colloid formation, were investigated by electrochemical techniques, a mercury pore sizer, N 2 adsorption [Brunauer‐Emmett‐Teller and Barrett‐Joyner‐Halenda] methods, and CO adsorption. The microstructure of the catalyst layer and its effect on polymer‐electrolyte fuel cell performance were affected by the contents of PFSI and carbon supports. The PFSI were distributed in the distinctive pores of 0.04 to 1.00 μm. Pore volume and pore diameter were primarily affected by the carbon supports. Carbon supports had a large pore volume with pore diameters less than 8 nm on the surface of the primary particles. Polymer‐electrolyte fuel cell performance predominantly increased with the specific volume of pores covered with the PFSI in the catalyst layer and with a decrease of the specific volume of pores less than 8 nm without PFSI on the carbon surface.

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Authors: Uchida, M., Fukuoka, Y., Sugawara, Y., Eda, N., & Ohta, A.
Affiliations: Technology Laboratory, Matsushita Battery Industrial Company, Limited, 1, Matsushita‐cho, Moriguchi, Osaka 570, Japan
ORCID: Uchida, Makoto
Ohta, Akira
Venue: Journal of The Electrochemical Society
Publisher: The Electrochemical Society
Published: 1996-07-01
Volume: 143
Issue: 7
Pages: 2245-2252
ISSN: 0013-4651 (ISSN-L)
1945-7111
DOI: 10.1149/1.1836988
OpenAlex: W1966315283
Cited by: 309
References: 0
Citations by year: 2026: 1 · 2025: 4 · 2024: 5 · 2023: 6 · 2022: 8 · 2021: 12 · 2020: 7 · 2019: 15 · 2018: 14 · 2017: 7 · 2016: 19 · 2015: 15 · 2014: 15 · 2013: 19 · 2012: 11
FWCI: 0.97
Type: journal article
Language: en
Open access: closed
Licence: iopscience.iop.org/page/copyright (vor, 8558 d)
iopscience.iop.org/info/page/text-and-data-mining (tdm, 8558 d)
Locations: Journal of The Electrochemical Society (publishedVersion)
Topics: Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Materials Science › Materials Chemistry › Advancements in Solid Oxide Fuel Cells
Keywords: proton exchange membrane fuel cells, catalyst layer microstructure, carbon support, platinum catalysts, perfluorosulfonate ionomers, pore size distribution, pore volume, specific surface area, fuel cell performance, CO adsorption

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Effects of Microstructure of Carbon Support in the Catalyst Layer on the Performance of Polymer‐Electrolyte Fuel Cells

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