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O 2 Reduction on an Ink‐Type Rotating Disk Electrode Using Pt Supported on High‐Area Carbons
Abstract
The kinetics of O 2 reduction has been examined on an ink‐type electrode made with Pt supported on high‐area carbon. Electrocatalysts with 5–40 mass % of Pt on Black Pearls, Vulcan XC‐72, and Shawinigan acetylene black carbons were used. Experiments were performed in 0.1 M solutions of H 2 SO 4 , H 3 PO 4 , HClO 4 , and NaOH. Kinetic parameters of O 2 reduction were found to be similar as on a smooth Pt surface. No influence of the type of carbon was observed. The mass activity of O 2 reduction was independent of Pt loading at low currents, but at high currents the mass activity decreased with an increase in Pt loading. It is suggested that mass‐transfer limitations are responsible for the different influence of Pt loading on mass activity at low and high currents. Reproducibility of the measurements on the ink electrode was satisfactory, and it is recommended for investigations of dispersed electrocatalysts.
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Citations
Cited by
Gasteiger, H. A., Kocha, S. S., Sompalli, B., & Wagner, F. T. (2005) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2004.06.021 · Cited by 4,876
Activation Energies for Oxygen Reduction on Platinum Alloys: Theory and Experiment
Anderson, A. B., Roques, J., Mukerjee, S., Murthi, V. S., Markovic, N. M., & Stamenkovic, V. (2005) · The Journal of Physical Chemistry B · doi:10.1021/jp047468z · Cited by 209
Controlled growth and shape formation of platinum nanoparticles and their electrochemical properties
Inaba, M., Ando, M., Hatanaka, A., Nomoto, A., Matsuzawa, K., Tasaka, A., Kinumoto, T., Iriyama, Y., & Ogumi, Z. (2006) · Electrochimica Acta · doi:10.1016/j.electacta.2006.03.094 · Cited by 107
Potential Shift for OH(ads) Formation on the Pt Skin on Pt[sub 3]Co(111) Electrodes in Acid
Roques, J., Anderson, A. B., Murthi, V. S., & Mukerjee, S. (2005) · Journal of The Electrochemical Society · doi:10.1149/1.1896328 · Cited by 61
Sahin, N. E., Napporn, T. W., Dubau, L., Kadirgan, F., Léger, J.-M., & Kokoh, K. B. (2017) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2016.09.026 · Cited by 47
Metadata
- Authors
- Gojković, S. L., Zečević, S. K., & Savinell, R. F.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 1998-11-01
- Volume
- 145
- Issue
- 11
- Pages
- 3713-3720
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W2111099931
- Cited by
- 170
- References
- 0
- FWCI
- 4.22
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: O 2 Reduction on an Ink‐Type Rotating Disk Electrode Using Pt Supported on High‐Area Carbons. https://app.cochat.ai/papers/10.1149/1.1838864
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- Gojković, S. L., Zečević, S. K., & Savinell, R. F. (1998). O 2 Reduction on an Ink‐Type Rotating Disk Electrode Using Pt Supported on High‐Area Carbons. Journal of The Electrochemical Society. https://doi.org/10.1149/1.1838864
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
