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A Point Defect Model for Anodic Passive Films: II . Chemical Breakdown and Pit Initiation
Open accessAbstract
The point defect model that was previously developed (1) to explain the growth kinetics of a passive film has been extended to account for chemical breakdown. This model provides quantitative explanations of the dependence of breakdown potential on halide concentration, and of the incubation time‐breakdown overpotential relationships that have been observed for iron and nickel in aqueous solutions. Limitations of the model are identified and discussed.
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Citations
Cited by
The history of the Point Defect Model for the passive state: A brief review of film growth aspects
Macdonald, D. D. (2011) · Electrochimica Acta · doi:10.1016/j.electacta.2010.11.005 · Cited by 1,117
Self-citationThin anodic oxide layers on aluminium and other valve metals: high field regime
Lohrengel, M. M. (1993) · Materials Science and Engineering: R: Reports · doi:10.1016/0927-796x(93)90005-n · Cited by 554
A Mathematical Model for the Lithium-Ion Negative Electrode Solid Electrolyte Interphase
Christensen, J., & Newman, J. (2004) · Journal of The Electrochemical Society · doi:10.1149/1.1804812 · Cited by 330
Metadata
- Authors
- Lin, L. F., Chao, C. Y., & Macdonald, D. D.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 1981-06-01
- Volume
- 128
- Issue
- 6
- Pages
- 1194-1198
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W1596628295
- Cited by
- 664
- References
- 0
- FWCI
- 6.13
- Type
- journal article
- Language
- en
- Open access
- bronze
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- CoChat. (2026). Citation check: A Point Defect Model for Anodic Passive Films: II . Chemical Breakdown and Pit Initiation. https://app.cochat.ai/papers/10.1149/1.2127592
- The paper
- Lin, L. F., Chao, C. Y., & Macdonald, D. D. (1981). A Point Defect Model for Anodic Passive Films: II . Chemical Breakdown and Pit Initiation. Journal of The Electrochemical Society. https://doi.org/10.1149/1.2127592
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
