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The Role of Hydrogen Peroxide in Oxygen Reduction at Platinum in H[sub 2]SO[sub 4] Solution
Abstract
The rotating disk electrode with a concentric ring is used to analyze the role of H 2 O 2 in the reduction of O 2 to H 2 O in acid solutions. No H 2 O 2 is formed as an intermediate in the reaction path of oxygen reduction to water. Only when the residual impurities from the not sufficiently purified solutions are adsorbed at the electrode does a parallel reaction path appear in which H 2 O 2 is formed as an intermediate that does not reduce further to H 2 O with any significant rate. The mechanism of O 2 reduction to H 2 O involves a first charge transfer step as rate‐controlling under Temkin conditions of adsorption.
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Cited by
Paulus, U. A., Schmidt, T. J., Gasteiger, H. A., & Behm, R. J. (2001) · Journal of Electroanalytical Chemistry · doi:10.1016/s0022-0728(00)00407-1 · Cited by 1,427
Doyle, R. L., Godwin, I. J., Brandon, M. P., & Lyons, M. E. G. (2013) · Physical Chemistry Chemical Physics · doi:10.1039/c3cp51213d · Cited by 600
Marković, N. M., Adžić, R. R., Cahan, B. D., & Yeager, E. B. (1994) · Journal of Electroanalytical Chemistry · doi:10.1016/0022-0728(94)03467-2 · Cited by 484
The oxygen reduction reaction on a Pt/carbon fuel cell catalyst in the presence of chloride anions
Schmidt, T. J., Paulus, U. A., Gasteiger, H. A., & Behm, R. J. (2001) · Journal of Electroanalytical Chemistry · doi:10.1016/s0022-0728(01)00499-5 · Cited by 481
Katsounaros, I., Schneider, W. B., Meier, J. C., Benedikt, U., Biedermann, P. U., Auer, A. A., & Mayrhofer, K. J. J. (2012) · Physical Chemistry Chemical Physics · doi:10.1039/c2cp40616k · Cited by 377
Metadata
- Authors
- Damjanovic, A., Genshaw, M. A., & Bockris, J. O.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 1967
- Volume
- 114
- Issue
- 5
- Pages
- 466
- ISSN
- 0013-4651 (ISSN-L)
- OpenAlex
- W2058497727
- Cited by
- 161
- References
- 0
- FWCI
- 4.62
- Type
- journal article
- Language
- en
- Open access
- closed
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- Damjanovic, A., Genshaw, M. A., & Bockris, J. O. (1967). The Role of Hydrogen Peroxide in Oxygen Reduction at Platinum in H[sub 2]SO[sub 4] Solution. Journal of The Electrochemical Society. https://doi.org/10.1149/1.2426629
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
