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Identification of the Source of Evolved Gas in Li-Ion Batteries Using [sup 13]C-labeled Solvents
Open accessAbstract
In order to elucidate the mechanism of gas evolution in lithium-ion batteries, we fabricated carbon– cells employing -labeled ethylene carbonate and diethyl carbonate as solvent components and then stored them at . The gas species evolved during storage tests were analyzed by gas chromatography/atomic emission detector to determine the isotopic ratio of and CO. The relative proportions of the derived from EC, DEC, and nonsolvent components were determined to be 52, 11, and 37%, respectively. The main source of was found to be EC. Further storage tests with either cathode or anode electrodes showed that the cathode components were a source of , but anode components were not. As for evolved CO, the main source was found to be EC. Moreover, we also examined the gas-evolution behavior on the initial charge. The evolved gas species were mainly composed of , , and CO. A minor amount of was also detected. From our isotopic analysis it was shown that was exclusively formed from EC, while derived from DEC. In the case of CO, EC and nonsolvent components were found to be its sources. CO derived from DEC was not detected.
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Citations
Cited by
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
A review of lithium ion battery failure mechanisms and fire prevention strategies
Wang, Q., Mao, B., Stoliarov, S. I., & Sun, J. (2019) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2019.03.002 · Cited by 1,755
Review on modeling of the anode solid electrolyte interphase (SEI) for lithium-ion batteries
Wang, A., Kadam, S., Li, H., Shi, S., & Qi, Y. (2018) · npj Computational Materials · doi:10.1038/s41524-018-0064-0 · Cited by 1,639
A review of hazards associated with primary lithium and lithium-ion batteries
Lisbona, D., & Snee, T. (2011) · Process Safety and Environmental Protection · doi:10.1016/j.psep.2011.06.022 · Cited by 701
A Review of Solid Electrolyte Interphase (SEI) and Dendrite Formation in Lithium Batteries
Li, B., Chao, Y., Li, M., Xiao, Y., Li, R., Yang, K., Cui, X., Xu, G., Li, L., Yang, C., et al. (2023) · Electrochemical Energy Reviews · doi:10.1007/s41918-022-00147-5 · Cited by 406
Metadata
- Authors
- Onuki, M., Kinoshita, S., Sakata, Y., Yanagidate, M., Otake, Y., Ue, M., & Deguchi, M.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2008
- Volume
- 155
- Issue
- 11
- Pages
- A794
- ISSN
- 0013-4651 (ISSN-L)
- OpenAlex
- W2107860851
- Cited by
- 211
- References
- 0
- FWCI
- 2.99
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Onuki, M., Kinoshita, S., Sakata, Y., Yanagidate, M., Otake, Y., Ue, M., & Deguchi, M. (2008). Identification of the Source of Evolved Gas in Li-Ion Batteries Using [sup 13]C-labeled Solvents. Journal of The Electrochemical Society. https://doi.org/10.1149/1.2969947
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