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Effect of Iron Substitution in the Electrochemical Performance of Na3V2(PO4)3as Cathode for Na-Ion Batteries
Open accessAbstract
Na 3 V 2-x Fe x (PO 4 ) 3 /C (0 ≤ x ≤ 0.5) samples were prepared by a simple sol-gel method. X-ray diffraction patterns revealed high purity and crystalline phosphate indexed in the R-3c space group. On increasing the iron content, the cell volume increases due to the slightly higher radius of Fe 3+ . Cyclic voltammetry showed two signals at ca. 3.5 and 4.0 V, which evidence a linear dependence of potential on the level of substitution. The appearance of the short plateau at ca. 4.0 V is closely related to the higher iron substitution levels. The evaluation of XPS and 57 Fe Mössbauer spectra of charged and discharged electrodes allow ascribing the 4.0 V plateau to V 4+ /V 5+ redox reaction and the extraction/insertion of extra sodium ions from octahedral M1 sites. Galvanostatic cycling showed capacity values as high as 115 mA h g −1 for samples with x = 0.1, 0.2, 0.3 and exceptional cyclability.
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Stamp, A., Lang, D. J., & Wäger, P. A. (2012) · Journal of Cleaner Production · doi:10.1016/j.jclepro.2011.10.026 · Cited by 151
Cited by
Recent Advances and Prospects of Cathode Materials for Sodium‐Ion Batteries
Xiang, X., Zhang, K., & Chen, J. (2015) · Advanced Materials · doi:10.1002/adma.201501527 · Cited by 1,160
Polyanion-type cathode materials for sodium-ion batteries
Jin, T., Li, H., Zhu, K., Wang, P.-F., Liu, P., & Jiao, L. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00846b · Cited by 908
Polyanion‐Type Electrode Materials for Sodium‐Ion Batteries
Ni, Q., Bai, Y., Wu, F., & Wu, C. (2017) · Advanced Science · doi:10.1002/advs.201600275 · Cited by 586
Na 3 V 2 (PO 4 ) 3 : an advanced cathode for sodium-ion batteries
Zhang, X., Rui, X., Chen, D., Tan, H., Yang, D., Huang, S., & Yu, Y. (2019) · Nanoscale · doi:10.1039/c8nr09391a · Cited by 336
Xu, G., Amine, R., Abouimrane, A., Che, H., Dahbi, M., Ma, Z., Saadoune, I., Alami, J., Mattis, W. L., Pan, F., et al. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201702403 · Cited by 287
Metadata
- Authors
- Aragón, M. J., Lavela, P., Ortiz, G. F., & Tirado, J. L.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2015
- Volume
- 162
- Issue
- 2
- Pages
- A3077-A3083
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W1983020788
- Cited by
- 170
- References
- 1
- FWCI
- 9.94
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Aragón, M. J., Lavela, P., Ortiz, G. F., & Tirado, J. L. (2015). Effect of Iron Substitution in the Electrochemical Performance of Na3V2(PO4)3as Cathode for Na-Ion Batteries. Journal of The Electrochemical Society. https://doi.org/10.1149/2.0151502jes
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