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A Near-Neutral Chloride Electrolyte for Electrically Rechargeable Zinc-Air Batteries
Open accessAbstract
Near-neutral electrolytes based on zinc chloride and ammonium chloride are examined for rechargeable zinc-air battery application. The effects of pH value, salt concentration, and polyethylene glycol and thiourea additives are investigated and a chloride electrolyte is developed. The reversible zinc deposition and zinc stripping processes are studied by cyclic voltammetry with rotating-disc electrode technique. The zinc anode and air cathode behaviors in near-neutral chloride electrolyte are characterized by quasi steady-state polarization and impedance spectroscopy. Prototyped zinc-air battery with near-neutral chloride electrolytes can sustain more than 1000 hours and hundreds of discharge-charge cycles with minimized zinc dendrite formation and no carbonate formation problem, under discharge-charge capacity ranging from 20 to 120 mAh. The near-neutral chloride electrolyte provides a safer and more robust alternative to traditional alkaline electrolyte for rechargeable zinc-air batteries.
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Citations
Cited by
Kundu, D., Adams, B. D., Duffort, V., Vajargah, S. H., & Nazar, L. F. (2016) · Nature Energy · doi:10.1038/nenergy.2016.119 · Cited by 3,124
Rechargeable Batteries for Grid Scale Energy Storage
Zhu, Z., Jiang, T., Ali, M., Meng, Y., Jin, Y., Cui, Y., & Chen, W. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00289 · Cited by 1,769
A rechargeable zinc-air battery based on zinc peroxide chemistry
Sun, W., Wang, F., Zhang, B., Zhang, M., Küpers, V., Ji, X., Theile, C., Bieker, P., Xu, K., Wang, C., et al. (2021) · Science · doi:10.1126/science.abb9554 · Cited by 1,082
Lee, B., Seo, H. R., Lee, H. R., Yoon, C. S., Kim, J. H., Chung, K. Y., Cho, B. W., & Oh, S. H. (2016) · ChemSusChem · doi:10.1002/cssc.201600702 · Cited by 489
Aqueous metal-air batteries: Fundamentals and applications
Liu, Q., Pan, Z., Wang, E., An, L., & Sun, G. (2020) · Energy Storage Materials · doi:10.1016/j.ensm.2019.12.011 · Cited by 417
Metadata
- Authors
- Thomas Goh, F. W., Liu, Z., Hor, T. S. A., Zhang, J., Ge, X., Zong, Y., Yu, A., & Khoo, W.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2014
- Volume
- 161
- Issue
- 14
- Pages
- A2080-A2086
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W2008436212
- Cited by
- 171
- References
- 0
- FWCI
- 2.83
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Thomas Goh, F. W., Liu, Z., Hor, T. S. A., Zhang, J., Ge, X., Zong, Y., Yu, A., & Khoo, W. (2014). A Near-Neutral Chloride Electrolyte for Electrically Rechargeable Zinc-Air Batteries. Journal of The Electrochemical Society. https://doi.org/10.1149/2.0311414jes
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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