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Heterodyne detection of the complete electric field of femtosecond four-wave mixing signals
Abstract
A novel optimized heterodyne method that recovers the complete electric field of any four-wave mixing signal at its point of origin is demonstrated. A tracer pulse is sent along the signal path and characterized at the sample by frequency-resolved optical gating. Spectral interferometry is used to determine the phase difference between the tracer and a reference pulse, the absorptive change in tracer phase in the sample, and the reference-signal phase difference. Together, these measurements allow calculation of the signal phase at the sample. The phase of three pulse-scattering signals from solutions of the infrared dye IR 144 in methanol determines the absolute signal-emission time within 0.5 fs.
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Citations
Cited by
Two-Dimensional Femtosecond Spectroscopy
Jonas, D. M. (2003) · Annual Review of Physical Chemistry · doi:10.1146/annurev.physchem.54.011002.103907 · Cited by 1,198
Self-citationMultidimensional Femtosecond Correlation Spectroscopies of Electronic and Vibrational Excitations
Mukamel, S. (2000) · Annual Review of Physical Chemistry · doi:10.1146/annurev.physchem.51.1.691 · Cited by 894
Coherent Two-Dimensional Optical Spectroscopy
Cho, M. (2008) · Chemical Reviews · doi:10.1021/cr078377b · Cited by 835
Exciton Coherence and Energy Transport in the Light-Harvesting Dimers of Allophycocyanin
Womick, J. M., & Moran, A. M. (2009) · The Journal of Physical Chemistry B · doi:10.1021/jp907644h · Cited by 119
Metadata
- Authors
- Gallagher, S. M., Albrecht, A. W., Hybl, J. D., Landin, B. L., Rajaram, B., & Jonas, D. M.
- Venue
- Journal of the Optical Society of America B
- Publisher
- Optica Publishing Group
- Published
- 1998-08-01
- Volume
- 15
- Issue
- 8
- Pages
- 2338
- ISSN
- 0740-3224 (ISSN-L)
- 1520-8540
- OpenAlex
- W2124442906
- Cited by
- 158
- References
- 0
- FWCI
- 8.59
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Heterodyne detection of the complete electric field of femtosecond four-wave mixing signals. https://app.cochat.ai/papers/10.1364/josab.15.002338
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- Gallagher, S. M., Albrecht, A. W., Hybl, J. D., Landin, B. L., Rajaram, B., & Jonas, D. M. (1998). Heterodyne detection of the complete electric field of femtosecond four-wave mixing signals. Journal of the Optical Society of America B. https://doi.org/10.1364/josab.15.002338
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