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Resonance lineshapes in two-dimensional Fourier transform spectroscopy
Open accessAbstract
We derive an analytical form for resonance lineshapes in two-dimensional (2D) Fourier transform spectroscopy. Our starting point is the solution of the optical Bloch equations for a two-level system in the 2D time domain. Application of the projection-slice theorem of 2D Fourier transforms reveals the form of diagonal and cross-diagonal slices in the 2D frequency data for arbitrary inhomogeneity. The results are applied in quantitative measurements of homogeneous and inhomogeneous broadening of multiple resonances in experimental data.
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Two-dimensional spectroscopy of electronic couplings in photosynthesis
Brixner, T., Stenger, J., Vaswani, H. M., Cho, M., Blankenship, R. E., & Fleming, G. R. (2005) · Nature · doi:10.1038/nature03429 · Cited by 1,241
Two-Dimensional Femtosecond Spectroscopy
Jonas, D. M. (2003) · Annual Review of Physical Chemistry · doi:10.1146/annurev.physchem.54.011002.103907 · Cited by 1,198
Cited by
Direct measurement of exciton valley coherence in monolayer WSe2
Hao, K., Moody, G., Wu, F., Dass, C. K., Xu, L., Chen, C.-H., Sun, L., Li, M.-Y., Li, L.-J., MacDonald, A. H., et al. (2016) · Nature Physics · doi:10.1038/nphys3674 · Cited by 317
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Metadata
- Authors
- Siemens, M. E., Moody, G., Li, H., Bristow, A. D., & Cundiff, S. T.
- Venue
- Optics Express
- Publisher
- Optica Publishing Group
- Published
- 2010-08-02
- Volume
- 18
- Issue
- 17
- Pages
- 17699
- ISSN
- 1094-4087 (ISSN-L)
- OpenAlex
- W2085416858
- Cited by
- 178
- References
- 2
- FWCI
- 3.62
- Type
- journal article
- Language
- en
- Open access
- gold
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- Siemens, M. E., Moody, G., Li, H., Bristow, A. D., & Cundiff, S. T. (2010). Resonance lineshapes in two-dimensional Fourier transform spectroscopy. Optics Express. https://doi.org/10.1364/oe.18.017699
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