The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Tunable two-dimensional femtosecond spectroscopy
Abstract
We have developed a two-dimensional (2D) Fourier-transform femtosecond spectroscopy technique for the visible spectral region. Three-pulse photon echo signals are generated in a phase-matched noncollinear four-wave mixing box geometry that employs a 3-kHz repetition-rate laser system and optical parametric amplification. Nonlinear signals are fully characterized in amplitude and phase by spectral interferometry. Unlike for previous setups, we achieve long-term phase stability by employing diffractive optics and interferometric accuracy of excitation-pulse time delays by using movable glass wedges. As an example of this technique, 2D correlation and relaxation spectra at 600 nm are shown for a solution of Nile Blue dye in acetonitrile.
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Citations
Cites
Two-Dimensional Femtosecond Spectroscopy
Jonas, D. M. (2003) · Annual Review of Physical Chemistry · doi:10.1146/annurev.physchem.54.011002.103907 · Cited by 1,198
Cited by
Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems
Engel, G. S., Calhoun, T. R., Read, E. L., Ahn, T.-K., Mančal, T., Cheng, Y.-C., Blankenship, R. E., & Fleming, G. R. (2007) · Nature · doi:10.1038/nature05678 · Cited by 3,315
Self-citationTwo-dimensional spectroscopy of electronic couplings in photosynthesis
Brixner, T., Stenger, J., Vaswani, H. M., Cho, M., Blankenship, R. E., & Fleming, G. R. (2005) · Nature · doi:10.1038/nature03429 · Cited by 1,241
Self-citationCoherent Two-Dimensional Optical Spectroscopy
Cho, M. (2008) · Chemical Reviews · doi:10.1021/cr078377b · Cited by 835
Quantum coherence in photosynthesis for efficient solar-energy conversion
Romero, E., Augulis, R., Novoderezhkin, V. I., Ferretti, M., Thieme, J., Zigmantas, D., & van Grondelle, R. (2014) · Nature Physics · doi:10.1038/nphys3017 · Cited by 594
Ultrafast Spectroscopy: State of the Art and Open Challenges
Maiuri, M., Garavelli, M., & Cerullo, G. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.9b10533 · Cited by 460
Metadata
- Authors
- Brixner, T., Stiopkin, I. V., & Fleming, G. R.
- Venue
- Optics Letters
- Publisher
- Optica Publishing Group
- Published
- 2004-04-15
- Volume
- 29
- Issue
- 8
- Pages
- 884
- ISSN
- 0146-9592 (ISSN-L)
- 1539-4794
- OpenAlex
- W2029357974
- Cited by
- 241
- References
- 1
- FWCI
- 7.58
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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