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Aerosol- and updraft-limited regimes of cloud droplet formation: influence of particle number, size and hygroscopicity on the activation of cloud condensation nuclei (CCN)

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Reutter, P., Su, H., Trentmann, J., Simmel, M., Rose, D., Gunthe, S. S., Wernli, H., Andreae, M. O., Pöschl, U.·2009·Atmospheric Chemistry and Physics

Abstract

Abstract. We have investigated the formation of cloud droplets under pyro-convective conditions using a cloud parcel model with detailed spectral microphysics and with the κ-Köhler model approach for efficient and realistic description of the cloud condensation nucleus (CCN) activity of aerosol particles. Assuming a typical biomass burning aerosol size distribution (accumulation mode centred at 120 nm), we have calculated initial cloud droplet number concentrations (NCD) for a wide range of updraft velocities (w=0.25–20 m s−1) and aerosol particle number concentrations (NCN=200–105 cm−3) at the cloud base. Depending on the ratio between updraft velocity and particle number concentration (w/NCN), we found three distinctly different regimes of CCN activation and cloud droplet formation: (1) An aerosol-limited regime that is characterized by high w/NCN ratios (>≈10−3 m s−1 cm3), high maximum values of water vapour supersaturation (Smax>≈0.5%), and high activated fractions of aerosol particles (NCN/NCN>≈90%). In this regime NCD is directly proportional to NCN and practically independent of w. (2) An updraft-limited regime that is characterized by low w/NCN ratios (

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Metadata

Authors
Reutter, P., Su, H., Trentmann, J., Simmel, M., Rose, D., Gunthe, S. S., Wernli, H., Andreae, M. O., & Pöschl, U.
Venue
Atmospheric Chemistry and Physics
Published
2009-09-24
Volume
9
Issue
18
Pages
7067-7080
ISSN
  • 1680-7316 (ISSN-L)
  • 1680-7324
OpenAlex
W2096462582
Cited by
346
References
1
FWCI
13.12
Type
journal article
Language
en
Open access
gold

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CoChat. (2026). Citation check: Aerosol- and updraft-limited regimes of cloud droplet formation: influence of particle number, size and hygroscopicity on the activation of cloud condensation nuclei (CCN). https://app.cochat.ai/papers/10.5194/acp-9-7067-2009
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Reutter, P., Su, H., Trentmann, J., Simmel, M., Rose, D., Gunthe, S. S., Wernli, H., Andreae, M. O., & Pöschl, U. (2009). Aerosol- and updraft-limited regimes of cloud droplet formation: influence of particle number, size and hygroscopicity on the activation of cloud condensation nuclei (CCN). Atmospheric Chemistry and Physics. https://doi.org/10.5194/acp-9-7067-2009

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