Study on Mode II Interfacial Fracture Toughness and Self‐Healing Efficiency of Self‐Healing Carbon Fiber Reinforced Polymer/Polyvinyl Chloride Foam Composite Sandwich Structures
Abstract
Self‐healing adhesive films (SHAFs) by embedding microcapsules containing epoxy and microcapsules containing hardener within an adhesive matrix are developed in this study. These SHAFs are engineered into carbon fiber reinforced polymer (CFRP)‐to‐ polyvinyl chloride (PVC) foam interfaces in composite sandwich structures to enable simultaneous interfacial toughening and autonomous crack repair. The effect of microcapsule content on mode II interfacial fracture toughness and self‐healing efficiency is studied using end‐notched flexure tests. The results demonstrate that the SHAFs containing 18.75 wt% microcapsules lead to a remarkable 103.95% improvement in mode II interfacial fracture toughness compared to conventional CFRP/PVC composite sandwich structures without the SHAFs, while also achieving a healing efficiency of 69.95%. A comprehensive analysis of crack deflection, microcapsule rupture‐triggered healing agent release, and interfacial rebonding mechanisms demonstrates the synergistic toughening‐healing behavior. This work establishes a scalable strategy for engineering high‐performance self‐healing composite sandwiches with dual functionality.
Integrity signals
Registry
Cites
Statistics
Claims the paper makes
Cites
Zhu, D. Y., Rong, M. Z., & Zhang, M. Q. (2015) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2015.07.002 · Cited by 634 · see citing works
Performance of self-healing epoxy with microencapsulated healing agent and shape memory alloy wires
Kirkby, E. L., Michaud, V. J., Månson, J.-A. E., Sottos, N. R., & White, S. R. (2009) · Polymer · doi:10.1016/j.polymer.2009.05.014 · Cited by 186 · see citing works
Review of z-pinned laminates and sandwich composites
Mouritz, A. P. (2020) · Composites Part A Applied Science and Manufacturing · doi:10.1016/j.compositesa.2020.106128 · Cited by 183 · see citing works
Mode II fracture testing of composites: a new look at an old problem
Blackman, B. R. K., Brunner, A. J., & Williams, J. G. (2006) · Engineering Fracture Mechanics · doi:10.1016/j.engfracmech.2006.05.022 · Cited by 182 · see citing works
Mechanical properties balance in novel Z-pinned sandwich panels: Out-of-plane properties
Marasco, A. I., Cartié, D., Partridge, I. K., et al. (2005) · Composites Part A Applied Science and Manufacturing · doi:10.1016/j.compositesa.2005.03.029 · Cited by 125 · see citing works
Microvascular based self-healing polymeric foam
Patrick, J. F., Sottos, N. R., & White, S. R. (2012) · Polymer · doi:10.1016/j.polymer.2012.07.021 · Cited by 90 · see citing works
State of the art review on mechanical properties of sandwich composite structures
Patekar, V., & Kale, K. B. (2022) · Polymer Composites · doi:10.1002/pc.26989 · Cited by 85 · see citing works
Sun, Z. G., Chen, H., Song, Z., et al. (2021) · Composites Part A Applied Science and Manufacturing · doi:10.1016/j.compositesa.2021.106289 · Cited by 84 · see citing works
Autonomic Healing of Carbon Fiber/Epoxy Interfaces
Jones, A. R., Cintora, A., White, S. R., et al. (2014) · ACS Applied Materials & Interfaces · doi:10.1021/am500536t · Cited by 82 · see citing works
Wear in-situ self-healing polymer composites incorporated with bifunctional microcapsules
Zhang, L., Wang, H., He, F., et al. (2021) · Composites Part B Engineering · doi:10.1016/j.compositesb.2021.109566 · Cited by 76 · see citing works
Influence of stitching on the fracture of stitched sandwich composites
Drake, D. A., Sullivan, R. W., Clay, S. B., et al. (2021) · Composites Part A Applied Science and Manufacturing · doi:10.1016/j.compositesa.2021.106383 · Cited by 50 · see citing works
Nano-reinforced polymeric healing agents for vascular self-repairing composites
Bekas, D. G., Baltzis, D., & Paipetis, A. S. (2016) · Materials & Design · doi:10.1016/j.matdes.2016.12.049 · Cited by 44 · see citing works
Ghazali, H., Ye, L., & Zhang, M. Q. (2017) · Composites Science and Technology · doi:10.1016/j.compscitech.2017.02.018 · Cited by 40 · see citing works
The influence of pin on the low-velocity impact performance of foam sandwich structure
Chen, J., Cheng, L., Sun, H., et al. (2022) · International Journal of Mechanical Sciences · doi:10.1016/j.ijmecsci.2022.108057 · Cited by 37 · see citing works
Ouyang, Q., Wang, X., & Liu, L. (2021) · Composites Science and Technology · doi:10.1016/j.compscitech.2021.109115 · Cited by 36 · see citing works
Mechanical properties and energy absorbing capabilities of Z-pinned aluminum foam sandwich
Raeisi, S., Kadkhodapour, J., & Tovar, A. (2019) · Composite Structures · doi:10.1016/j.compstruct.2019.01.095 · Cited by 30 · see citing works
Wu, Q. L., Li, Y., Chang, J. S., et al. (2024) · Composites Part B Engineering · doi:10.1016/j.compositesb.2024.112007 · Cited by 29 · see citing works
Self-citationEffects of stitching parameters on the mechanical properties of stitched sandwich panel structures
Ai, S., Chen, Y., & He, R. (2020) · Ceramics International · doi:10.1016/j.ceramint.2020.10.105 · Cited by 28 · see citing works
Highly tough 3D woven composite materials: Fracture characterization and toughening mechanisms
Xu, W., Zhang, S., Liu, W., et al. (2022) · Theoretical and Applied Fracture Mechanics · doi:10.1016/j.tafmec.2022.103734 · Cited by 28 · see citing works
Peng, A., Deng, J., Wu, D., et al. (2023) · Thin-Walled Structures · doi:10.1016/j.tws.2023.111155 · Cited by 28 · see citing works
Effect of tufting density and loop length on the crushing behaviour of tufted sandwich specimens
Hartley, J. W., Kratz, J., Ward, C., et al. (2016) · Composites Part B Engineering · doi:10.1016/j.compositesb.2016.12.037 · Cited by 27 · see citing works
Ostapiuk, M., Loureiro, M. V., Bienias, J., et al. (2020) · Composite Structures · doi:10.1016/j.compstruct.2020.113042 · Cited by 27 · see citing works
Farmand-Ashtiani, E., Cugnoni, J., & Botsis, J. (2012) · Composite Structures · doi:10.1016/j.compstruct.2012.08.059 · Cited by 23 · see citing works
Wang, Z., Li, Y., & Tu, H. (2022) · Composites Part A Applied Science and Manufacturing · doi:10.1016/j.compositesa.2022.107096 · Cited by 23 · see citing works
Self-citationChen, Q., Du, S., Jiang, Z., et al. (2020) · Polymer Composites · doi:10.1002/pc.25630 · Cited by 22 · see citing works
Özer, H., Kuzu, E., Özada, Ç., et al. (2021) · Construction and Building Materials · doi:10.1016/j.conbuildmat.2021.125303 · Cited by 22 · see citing works
3D printed continuous fibre composite repair of sandwich structures
Joosten, M. W., Neave, M. B., Rider, A. N., & Varley, R. J. (2022) · Composite Structures · doi:10.1016/j.compstruct.2022.115518 · Cited by 22 · see citing works
Impact response of composite sandwich structures with toughened matrices
Irven, G., Duncan, A. M., Whitehouse, A. D., et al. (2021) · Materials & Design · doi:10.1016/j.matdes.2021.109629 · Cited by 18 · see citing works
Zhao, L., Li, H., Qiao, Y., et al. (2022) · Journal of Applied Polymer Science · doi:10.1002/app.53458 · Cited by 18 · see citing works
Caprino, G., Durante, M., Leone, C., et al. (2014) · Composites Part B Engineering · doi:10.1016/j.compositesb.2014.10.042 · Cited by 16 · see citing works
Devaraj, S. J., & Kumar, A. A. J. (2022) · Polymer Composites · doi:10.1002/pc.26868 · Cited by 14 · see citing works
Li, L., Chuan, J., Shen, X., et al. (2023) · Composite Structures · doi:10.1016/j.compstruct.2023.116769 · Cited by 14 · see citing works
Tsai, S.-N., & Taylor, A. C. (2018) · Composite Structures · doi:10.1016/j.compstruct.2018.11.071 · Cited by 13 · see citing works
In-situ repair of composite sandwich structures using cyanoacrylates
Cullinan, J. F., Velut, P., Michaud, V. J., et al. (2016) · Composites Part A Applied Science and Manufacturing · doi:10.1016/j.compositesa.2016.04.029 · Cited by 12 · see citing works
Atar, H. A., Zarrebini, M., Hasani, H., et al. (2020) · Journal of Sandwich Structures & Materials · doi:10.1177/1099636219900343 · Cited by 12 · see citing works
Chen, C., Legrand, X., Hong, Y., et al. (2022) · Composite Structures · doi:10.1016/j.compstruct.2022.116594 · Cited by 12 · see citing works
Toughening of face-sheet core bonds in sandwich structures
Irven, G., Whitehouse, A. D., Carolan, D., et al. (2023) · Engineering Fracture Mechanics · doi:10.1016/j.engfracmech.2023.109498 · Cited by 12 · see citing works
Impact and CAI behavior of SGF mat filled sandwich panels made from foam core and FRP facesheet
Liang, W., Bonsu, A. O., Tang, X., et al. (2021) · Composites Communications · doi:10.1016/j.coco.2021.101000 · Cited by 11 · see citing works
Akdere, H. Ö., & Uzay, Ç. (2025) · Arabian Journal for Science and Engineering · doi:10.1007/s13369-025-10061-9 · Cited by 10 · see citing works
Wang, B., Luo, B., Qu, Y. D., et al. (2024) · Aerospace Science and Technology · doi:10.1016/j.ast.2024.108902 · Cited by 9 · see citing works
Thermoplastic foam injection moulding of sandwich structures with short fibre-reinforced skin layers
Loypetch, N., Tröltzsch, J., Nestler, D., et al. (2019) · Journal of Sandwich Structures & Materials · doi:10.1177/1099636219829423 · Cited by 8 · see citing works
Thermal stresses in the discrete joints of sandwiched structures
Wong, E. H. (2015) · Composite Structures · doi:10.1016/j.compstruct.2015.01.027 · Cited by 6 · see citing works
Wang, B., Tian, W., Wang, C., et al. (2025) · Polymer Composites · doi:10.1002/pc.29573 · Cited by 6 · see citing works
Peng, Y., Li, M., Yang, X., et al. (2025) · Thin-Walled Structures · doi:10.1016/j.tws.2025.113244 · Cited by 6 · see citing works
Study on Thermal Properties of Epoxy-Adhesive Film for Aluminum Sandwich Composite Structure
Oh, K., & Park, H. (2020) · International Journal of Aeronautical and Space Sciences · doi:10.1007/s42405-020-00315-1 · Cited by 4 · see citing works
Typical failure modes and corresponding repairing methods of woven lattice sandwich composites
Li, X., Shi, H., Bai, C., et al. (2024) · Polymer Composites · doi:10.1002/pc.28862 · Cited by 2 · see citing works
Flagged first, then by citations
Cited by
Sorted by citations
Asadpour, A., Salehi, M., & Eslami-Farsani, R. (2026) · Composites Part C: Open Access · doi:10.1016/j.jcomc.2026.100799
- Authors
- Wang, Z., Huang, Z., Zhang, Z., & Li, Y.
- Affiliations
- Tongji University (CN)
- Ningbo University of Technology (CN)
- Corresponding author
- Zhang, Zhongsen
- Li, Yan
- Venue
- Advanced Engineering Materials
- Publisher
- Wiley
- Published
- 2025-07-30
- Volume
- 27
- Issue
- 18
- ISSN
- 1438-1656 (ISSN-L)
- 1527-2648
- OpenAlex
- W4412740544
- Semantic Scholar
- 938f2af4060998efa666f622dcc8c72db5e48459
- Cited by
- 0
- References
- 46
- FWCI
- 0.00
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Advanced Engineering Materials (publishedVersion)
- Topics
- Physical Sciences › Materials Science › Polymers and Plastics › Polymer composites and self-healing
- Physical Sciences › Engineering › Mechanics of Materials › Mechanical Behavior of Composites
- Physical Sciences › Engineering › Mechanical Engineering › Epoxy Resin Curing Processes
- Keywords
- self-healing adhesives, microcapsules, carbon fiber reinforced polymer, polyvinyl chloride foam, sandwich structures, crack repair, end-notched flexure, crack deflection, interfacial toughening, healing efficiency
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
Are you an author, or do you see a problem with this page? Request a review