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Synthesis of Hierarchically Porous Carbon Monoliths with Highly Ordered Microstructure and Their Application in Rechargeable Lithium Batteries with High‐Rate Capability
Abstract
In this paper, we report on Li storage in hierarchically porous carbon monoliths with a relatively higher graphite‐like ordered carbon structure. Macroscopic carbon monoliths with both mesopores and macropores were successfully prepared by using meso‐/macroporous silica as a template and using mesophase pitch as a precursor. Owing to the high porosity (providing ionic transport channels) and high electronic conductivity (ca. 0.1 S cm–1), this porous carbon monolith with a mixed conducting 3D network shows a superior high‐rate performance if used as anode material in electrochemical lithium cells. A challenge for future research as to its applicability in batteries is the lowering of the irreversible capacity.
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Citations
Cited by
Chemistry and materials options of sustainable carbon materials made by hydrothermal carbonization
Titirici, M.-M., & Antonietti, M. (2010) · Chem. Soc. Rev. · doi:10.1039/b819318p · Cited by 1,255
Self-citationAdvanced carbon aerogels for energy applications
Biener, J., Stadermann, M., Suss, M., Worsley, M. A., Biener, M. M., Rose, K. A., & Baumann, T. F. (2011) · Energy & Environmental Science · doi:10.1039/c0ee00627k · Cited by 651
Mesoporous materials and electrochemistry
Walcarius, A. (2013) · Chemical Society Reviews · doi:10.1039/c2cs35322a · Cited by 623
Hollow Carbon-Nanotube/Carbon-Nanofiber Hybrid Anodes for Li-Ion Batteries
Chen, Y., Li, X., Park, K., Song, J., Hong, J., Zhou, L., Mai, Y.-W., Huang, H., & Goodenough, J. B. (2013) · Journal of the American Chemical Society · doi:10.1021/ja408421n · Cited by 444
Xing, Z., Ju, Z., Zhao, Y., Wan, J., Zhu, Y., Qiang, Y., & Qian, Y. (2016) · Scientific Reports · doi:10.1038/srep26146 · Cited by 435
Metadata
- Authors
- Hu, Y. ‐., Adelhelm, P., Smarsly, B. M., Hore, S., Antonietti, M., & Maier, J.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2007-07-12
- Volume
- 17
- Issue
- 12
- Pages
- 1873-1878
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2123916020
- Cited by
- 707
- References
- 0
- FWCI
- 24.25
- Type
- journal article
- Language
- en
- Open access
- closed
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- Hu, Y. ‐., Adelhelm, P., Smarsly, B. M., Hore, S., Antonietti, M., & Maier, J. (2007). Synthesis of Hierarchically Porous Carbon Monoliths with Highly Ordered Microstructure and Their Application in Rechargeable Lithium Batteries with High‐Rate Capability. Advanced Functional Materials. https://doi.org/10.1002/adfm.200601152
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