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Sustained Lithium‐Storage Performance of Hierarchical, Nanoporous Anatase TiO2 at High Rates: Emphasis on Interfacial Storage Phenomena
Abstract
A hierarchical, nanoporous TiO 2 structure is successfully prepared by a simple in situ hydrolysis method. Used as an anode material, it achieves a sustained high lithium storage performance especially at high charge/discharge rates due to its substantially high surface area. The material shows two different major storage modes: a) bulk insertion, and b) pseudo‐capacitive interfacial storage, which is responsible for 64% of the total capacity. In order to kinetically emphasize the interfacial storage even further, we cycle the material directly at high rates, giving 302 mA h g−1 and 200 mA h g−1 of fully reversible discharge capacity at charge/discharge rates of 1 C and 5 C with very high cycle stability. We propose an overall view on the different Li insertion mechanisms of the high‐surface‐area nanoporous TiO 2 and emphasize the importance of interfacial storage for electrode applications in Li‐ion batteries.
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Sing, K. S. W. (1985) · Pure and Applied Chemistry · doi:10.1351/pac198557040603 · Cited by 24,485
On a theory of the van der waals adsorption of gases
Brunauer, S., Deming, L. S., Deming, W. E., & Teller, E. (1940) · Journal of the American Chemical Society · doi:10.1021/ja01864a025 · Cited by 4,829
Cited by
Exploring Anomalous Charge Storage in Anode Materials for Next-Generation Li Rechargeable Batteries
Kim, H., Choi, W., Yoon, J., Um, J. H., Lee, W., Kim, J., Cabana, J., & Yoon, W.-S. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00618 · Cited by 527
Research Progress on Negative Electrodes for Practical Li‐Ion Batteries: Beyond Carbonaceous Anodes
Aravindan, V., Lee, Y., & Madhavi, S. (2015) · Advanced Energy Materials · doi:10.1002/aenm.201402225 · Cited by 462
Shin, J.-Y., Joo, J. H., Samuelis, D., & Maier, J. (2012) · Chemistry of Materials · doi:10.1021/cm2031009 · Cited by 401
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Metadata
- Authors
- Shin, J., Samuelis, D., & Maier, J.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2011-08-03
- Volume
- 21
- Issue
- 18
- Pages
- 3464-3472
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W1980747973
- Cited by
- 587
- References
- 2
- FWCI
- 31.42
- Type
- journal article
- Language
- en
- Open access
- closed
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- Shin, J., Samuelis, D., & Maier, J. (2011). Sustained Lithium‐Storage Performance of Hierarchical, Nanoporous Anatase TiO2 at High Rates: Emphasis on Interfacial Storage Phenomena. Advanced Functional Materials. https://doi.org/10.1002/adfm.201002527
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