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Morphological Control for High Performance, Solution‐Processed Planar Heterojunction Perovskite Solar Cells

Eperon, Giles E., Burlakov, Victor M., Docampo, Pablo, Goriely, Alain, Snaith, Henry J.·2014·Advanced Functional Materials

Abstract

Organometal trihalide perovskite based solar cells have exhibited the highest efficiencies to‐date when incorporated into mesostructured composites. However, thin solid films of a perovskite absorber should be capable of operating at the highest efficiency in a simple planar heterojunction configuration. Here, it is shown that film morphology is a critical issue in planar heterojunction CH 3 NH 3 PbI 3‐xClx solar cells. The morphology is carefully controlled by varying processing conditions, and it is demonstrated that the highest photocurrents are attainable only with the highest perovskite surface coverages. With optimized solution based film formation, power conversion efficiencies of up to 11.4% are achieved, the first report of efficiencies above 10% in fully thin‐film solution processed perovskite solar cells with no mesoporous layer.

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Metadata

Authors
Eperon, G. E., Burlakov, V. M., Docampo, P., Goriely, A., & Snaith, H. J.
Venue
Advanced Functional Materials
Publisher
Wiley
Published
2013-09-09
Volume
24
Issue
1
Pages
151-157
ISSN
  • 1616-301X (ISSN-L)
  • 1616-3028
OpenAlex
W2091471276
Cited by
1,982
References
1
FWCI
162.56
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Morphological Control for High Performance, Solution‐Processed Planar Heterojunction Perovskite Solar Cells. https://app.cochat.ai/papers/10.1002/adfm.201302090
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Eperon, G. E., Burlakov, V. M., Docampo, P., Goriely, A., & Snaith, H. J. (2014). Morphological Control for High Performance, Solution‐Processed Planar Heterojunction Perovskite Solar Cells. Advanced Functional Materials. https://doi.org/10.1002/adfm.201302090

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