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Novel Composites of α‐Fe2O3 Tetrakaidecahedron and Graphene Oxide as an Effective Photoelectrode with Enhanced Photocurrent Performances
Abstract
Novel composites composed of α‐Fe 2 O 3 tetrakaidecahedrons and graphene oxide have been easily fabricated and demonstrated to be efficient photoelectrodes for photoelectrochemical water splitting reaction with superior photocurrent response. α‐Fe 2 O 3 tetrakaidecahedrons are facilely synthesized in a green manner without any organic additives and then modified with graphene oxide. The morphological and structural properties of α‐Fe 2 O 3/graphene composite are intensively investigated by several means, such as X‐ray diffraction, field‐emission scanning electron microscope, transmission electron microscope, X‐ray photoelectron spectroscopy, Fourier Transform infrared spectroscopy, and Raman spectroscopy. The tetrakaidecahedronal hematite particles have been indicated to be successfully coupled with graphene oxide. Systematical photoelectrochemical and impedance spectroscopy measurements have been carried out to investigate the favorable performance of α‐Fe 2 O 3/graphene composites, which are found to be effective photoanodes with rapid, steady, and reproducible feature. The coupling of graphene with α‐Fe 2 O 3 particles has greatly enhanced the photoelectrochemical performance, resulting in higher photocurrent and lower onset potential than that of pure α‐Fe 2 O 3. This investigation has provided a feasible method to synthesize α‐Fe 2 O 3 tetrakaidecahedron and fabricate an efficient α‐Fe 2 O 3/graphene photoelectrode for photoelectrochemical water oxidation, suggesting a promising route to design noble metal free semiconductor/graphene photocatalysts.
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Liu, J., Bai, H., Wang, Y., Liu, Z., Zhang, X., & Sun, D. D. (2010) · Advanced Functional Materials · doi:10.1002/adfm.201001391 · Cited by 776
Cited by
Crystal Facet Engineering of Photoelectrodes for Photoelectrochemical Water Splitting
Wang, S., Liu, G., & Wang, L. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00584 · Cited by 847
Li, C., Cao, Q., Wang, F., Xiao, Y., Li, Y., Delaunay, J.-J., & Zhu, H. (2018) · Chemical Society Reviews · doi:10.1039/c8cs00067k · Cited by 494
Liu, W., Liu, H., Dang, L., Zhang, H., Wu, X., Yang, B., Li, Z., Zhang, X., Lei, L., & Jin, S. (2017) · Advanced Functional Materials · doi:10.1002/adfm.201603904 · Cited by 357
Xin, S., Tang, Y., Jia, B., Zhang, Z., Li, C., Bao, R., Li, C., Yi, J., Wang, J., & Ma, T. (2023) · Advanced Functional Materials · doi:10.1002/adfm.202305243 · Cited by 266
Metadata
- Authors
- Liu, S., Zheng, L., Yu, P., Han, S., & Fang, X.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2016-03-15
- Volume
- 26
- Issue
- 19
- Pages
- 3331-3339
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2300305241
- Cited by
- 230
- References
- 1
- FWCI
- 7.42
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, S., Zheng, L., Yu, P., Han, S., & Fang, X. (2016). Novel Composites of α‐Fe2O3 Tetrakaidecahedron and Graphene Oxide as an Effective Photoelectrode with Enhanced Photocurrent Performances. Advanced Functional Materials. https://doi.org/10.1002/adfm.201505554
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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