Cited by 208Polymer composites and self-healingAdvanced Polymer Synthesis and CharacterizationEpoxy Resin Curing Processes

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Mechanically Robust, Self‐Healable, and Highly Stretchable “Living” Crosslinked Polyurethane Based on a Reversible CC Bond

Zhang, Ze Ping, Rong, Min Zhi, Zhang, Ming Qiu·2018·Advanced Functional Materials

DOI 10.1002/adfm.201706050

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Abstract

Stimuli‐responsive polymers built by reversible covalent bonds used to possess unbalanced mechanical properties. Here, a crosslinked polyurethane containing aromatic pinacol as a novel reversible CC bond provider is synthesized, whose tensile strength and failure strain are tunable from 27.3 MPa to as high as 115.2 MPa and from 324% to 1501%, respectively, owing to the relatively high bond energy of the CC bond of pinacol as well as the hydrogen bond between hard segments and semicrystalline soft segments. Moreover, the dynamic equilibrium of pinacol enables self‐healing and recycling of the polymer. Interestingly, the dynamic exchange among macromolecules, for the first time, successfully cooperates with solid‐state drawing that applies to thermoplastics, realizing strengthening of thermoset. Meanwhile, the radicals derived from homolysis of pinacol can repeatedly initiate polymerization of vinyl monomers. The fruitful outcomes of this work may create a series of promising new techniques.

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Authors: Zhang, Z. P., Rong, M. Z., & Zhang, M. Q.
Affiliations: Sun Yat-sen University (CN)
Corresponding author: Rong, Min Zhi
Zhang, Ming Qiu
ORCID: Zhang, Ze Ping
Rong, Min Zhi
Zhang, Ming Qiu
Venue: Advanced Functional Materials
Publisher: Wiley
Published: 2018-01-16
Volume: 28
Issue: 11
ISSN: 1616-301X (ISSN-L)
1616-3028
DOI: 10.1002/adfm.201706050
OpenAlex: W2783944931
Cited by: 208
References: 46
Citations by year: 2026: 7 · 2025: 11 · 2024: 15 · 2023: 28 · 2022: 34 · 2021: 23 · 2020: 41 · 2019: 34 · 2018: 15
FWCI: 14.10
Type: journal article
Language: en
Open access: closed
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Advanced Functional Materials (publishedVersion)
Funders: National Natural Science Foundation of China (51673219, 51333008)
Topics: Physical Sciences › Materials Science › Polymers and Plastics › Polymer composites and self-healing
Physical Sciences › Chemistry › Organic Chemistry › Advanced Polymer Synthesis and Characterization
Physical Sciences › Materials Science › Polymers and Plastics › Epoxy Resin Curing Processes
Keywords: crosslinked polyurethane, pinacol, self-healing polymers, stimuli-responsive polymers, stretchable polymers, mechanical properties, hydrogen bonding, solid-state drawing, radical polymerization, vinyl polymerization, polymer recycling

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Mechanically Robust, Self‐Healable, and Highly Stretchable “Living” Crosslinked Polyurethane Based on a Reversible CC Bond

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