The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Fe, Cu‐Coordinated ZIF‐Derived Carbon Framework for Efficient Oxygen Reduction Reaction and Zinc–Air Batteries
Abstract
Zeolitic imidazole frameworks (ZIFs) offer rich platforms for rational design and construction of high‐performance nonprecious‐metal oxygen reduction reaction (ORR) catalysts owing to their flexibility, hierarchical porous structures, and high surface area. Herein, an Fe, Cu‐coordinated ZIF‐derived carbon framework (Cu@Fe‐N‐C) with a well‐defined morphology of truncated rhombic dodecahedron is facilely prepared by introducing Fe 2+ and Cu 2+ during the growth of ZIF‐8, followed by pyrolysis. The obtained Cu@Fe‐N‐C, with bimetallic active sites, large surface area, high nitrogen doping level, and conductive carbon frameworks, exhibits excellent ORR performance. It displays 50 mV higher half‐wave potential (0.892 V) than that of Pt catalysts in an alkaline medium and comparable performance to Pt catalysts in an acidic medium. In addition, it also has excellent durability and methanol resistance ability in both acidic and alkaline solutions, which makes it one of the best Pt‐free catalysts reported to date for ORR. Impressively, when being employed as a cathode catalyst in zinc–air batteries, Cu@Fe‐N‐C presents a higher peak power density of 92 mW cm−2 than that of Pt/C (74 mW cm−2) as well as excellent durability.
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Cites
Origin of the Overpotential for Oxygen Reduction at a Fuel-Cell Cathode
Nørskov, J. K., Rossmeisl, J., Logadottir, A., Lindqvist, L., Kitchin, J. R., Bligaard, T., & Jónsson, H. (2004) · The Journal of Physical Chemistry B · doi:10.1021/jp047349j · Cited by 13,153
High-Performance Electrocatalysts for Oxygen Reduction Derived from Polyaniline, Iron, and Cobalt
Wu, G., More, K. L., Johnston, C. M., & Zelenay, P. (2011) · Science · doi:10.1126/science.1200832 · Cited by 3,984
Recent Advances in Electrocatalysts for Oxygen Reduction Reaction
Shao, M., Chang, Q., Dodelet, J.-P., & Chenitz, R. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00462 · Cited by 3,903
Cheng, H., Li, M., Su, C., Li, N., & Liu, Z. (2017) · Advanced Functional Materials · doi:10.1002/adfm.201701833 · Cited by 384
Cited by
Cobalt single atom site isolated Pt nanoparticles for efficient ORR and HER in acid media
Liang, L., Jin, H., Zhou, H., Liu, B., Hu, C., Chen, D., Wang, Z., Hu, Z., Zhao, Y., Li, H.-W., et al. (2021) · Nano Energy · doi:10.1016/j.nanoen.2021.106221 · Cited by 360
Self-citationAo, X., Zhang, W., Zhao, B., Ding, Y., Nam, G., Soule, L., Abdelhafiz, A., Wang, C., & Liu, M. (2020) · Energy & Environmental Science · doi:10.1039/d0ee00832j · Cited by 330
He, T., Zhang, Y., Chen, Y., Zhang, Z., Wang, H., Hu, Y., Liu, M., Pao, C.-W., Chen, J.-L., Chang, L. Y., et al. (2019) · Journal of Materials Chemistry A · doi:10.1039/c9ta05981d · Cited by 104
Hao, Y.-R., Xue, H., Sun, J., Guo, N., Song, T., Sun, J., & Wang, Q. (2021) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.1c14387 · Cited by 58
Metadata
- Authors
- Wang, Z., Jin, H., Meng, T., Liao, K., Meng, W., Yang, J., He, D., Xiong, Y., & Mu, S.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2018-08-02
- Volume
- 28
- Issue
- 39
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2885063588
- Cited by
- 498
- References
- 4
- FWCI
- 14.36
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, Z., Jin, H., Meng, T., Liao, K., Meng, W., Yang, J., He, D., Xiong, Y., & Mu, S. (2018). Fe, Cu‐Coordinated ZIF‐Derived Carbon Framework for Efficient Oxygen Reduction Reaction and Zinc–Air Batteries. Advanced Functional Materials. https://doi.org/10.1002/adfm.201802596
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