The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Biomass Valorization via Paired Electrosynthesis Over Vanadium Nitride‐Based Electrocatalysts
Abstract
Paired electrosynthesis is a promising technology with the potential to generate value‐added products at both electrodes in a cost‐effective manner. Herein, 3D vanadium nitride (VN) and Pd/VN hollow nanospheres are successfully fabricated and coupled to carry out simultaneous electrocatalytic oxidation (ECO) and electrocatalytic hydrogenation (ECH) of 5‐hydroxymethylfurfural (HMF) into 2, 5‐furandicarboxylic acid (FDCA) and 2,5‐bishydroxymethyl‐tetrahydrofuran (DHMTHF), respectively. VN shows excellent ECO performance with high HMF conversion (≥98%), FDCA selectivity (≥96%), and faradaic efficiency (≥84%) after a stability test, and Pd/VN achieves high ECH selectivity for DHMTHF at ≥88% and an HMF conversion of ≥90%, with a faradaic efficiency of ≥86%. VN and Pd/VN incorporated into a membrane electrode assembly in a paired electrolysis system shows potential for large‐scale biomass conversion and upgrading. Theoretical calculations reveal that the higher performance of VN for the production of ECO can be attributed to its lower d‐band center level relative to the Fermi level compared to that of V 2 O 5, which favors HMF chemisorption and activation. This study paves the way for developing paired electrosynthesis technologies with the potential for biomass utilization and energy conversion.
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Cites
Chen, Z., Song, Y., Cai, J., Zheng, X., Han, D., Wu, Y., Zang, Y., Niu, S., Liu, Y., Zhu, J., et al. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201801834 · Cited by 1,075
Cited by
Xu, C., Paone, E., Rodríguez-Padrón, D., Luque, R., & Mauriello, F. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00041h · Cited by 1,042
Yang, Y., & Mu, T. (2021) · Green Chemistry · doi:10.1039/d1gc00914a · Cited by 539
Recent Advancements in Electrochemical Hydrogen Production via Hybrid Water Splitting
Qian, Q., Zhu, Y., Ahmad, N., Feng, Y., Zhang, H., Cheng, M., Liu, H., Xiao, C., Zhang, G., & Xie, Y. (2024) · Advanced Materials · doi:10.1002/adma.202306108 · Cited by 399
Pang, X., Bai, H., Zhao, H., Fan, W., & Shi, W. (2022) · ACS Catalysis · doi:10.1021/acscatal.1c04880 · Cited by 285
Electrochemical hydrogenation and oxidation of organic species involving water
Liu, C., Chen, F., Zhao, B.-H., Wu, Y., & Zhang, B. (2024) · Nature Reviews Chemistry · doi:10.1038/s41570-024-00589-z · Cited by 269
Metadata
- Authors
- Li, S., Sun, X., Yao, Z., Zhong, X., Cao, Y., Liang, Y., Wei, Z., Deng, S., Zhuang, G., Li, X., & Wang, J.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2019-08-15
- Volume
- 29
- Issue
- 42
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2968672313
- Cited by
- 226
- References
- 1
- FWCI
- 6.30
- Type
- journal article
- Language
- en
- Open access
- closed
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- Li, S., Sun, X., Yao, Z., Zhong, X., Cao, Y., Liang, Y., Wei, Z., Deng, S., Zhuang, G., Li, X., & Wang, J. (2019). Biomass Valorization via Paired Electrosynthesis Over Vanadium Nitride‐Based Electrocatalysts. Advanced Functional Materials. https://doi.org/10.1002/adfm.201904780
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