The DOI matches its Crossref record; 38 of the 38 references it cites were found in a registry or an index.
Antifreezing Hydrogel with High Zinc Reversibility for Flexible and Durable Aqueous Batteries by Cooperative Hydrated Cations
Open accessAbstract
Hydrogels are widely used in flexible aqueous batteries due to their liquid‐like ion transportation abilities and solid‐like mechanical properties. Their potential applications in flexible and wearable electronics introduce a fundamental challenge: how to lower the freezing point of hydrogels to preserve these merits without sacrificing hydrogels' basic advantages in low cost and high safety. Moreover, zinc as an ideal anode in aqueous batteries suffers from low reversibility because of the formation of insulative byproducts, which is mainly caused by hydrogen evolution via extensive hydration of zinc ions. This, in principle, requires the suppression of hydration, which induces an undesirable increase in the freezing point of hydrogels. Here, it is demonstrated that cooperatively hydrated cations, zinc and lithium ions in hydrogels, are very effective in addressing the above challenges. This simple but unique hydrogel not only enables a 98% capacity retention upon cooling down to −20 °C from room temperature but also allows a near 100% capacity retention with >99.5% Coulombic efficiency over 500 cycles at −20 °C. In addition, the strengthened mechanical properties of the hydrogel under subzero temperatures result in excellent durability under various harsh deformations after the freezing process.
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Cites
Highly reversible zinc metal anode for aqueous batteries
Wang, F., Borodin, O., Gao, T., Fan, X., Sun, W., Han, F., Faraone, A., Dura, J. A., Xu, K., & Wang, C. (2018) · Nature Materials · doi:10.1038/s41563-018-0063-z · Cited by 3,305
Kundu, D., Adams, B. D., Duffort, V., Vajargah, S. H., & Nazar, L. F. (2016) · Nature Energy · doi:10.1038/nenergy.2016.119 · Cited by 3,124
Reversible aqueous zinc/manganese oxide energy storage from conversion reactions
Pan, H., Shao, Y., Yan, P., Cheng, Y., Han, K. S., Nie, Z., Wang, C., Yang, J., Li, X., Bhattacharya, P., et al. (2016) · Nature Energy · doi:10.1038/nenergy.2016.39 · Cited by 3,066
Recent Advances in Aqueous Zinc-Ion Batteries
Fang, G., Zhou, J., Pan, A., & Liang, S. (2018) · ACS Energy Letters · doi:10.1021/acsenergylett.8b01426 · Cited by 2,258
Recent Advances in Zn‐Ion Batteries
Song, M., Tan, H., Chao, D., & Fan, H. J. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201802564 · Cited by 2,196
Wan, F., Zhang, L., Dai, X., Wang, X., Niu, Z., & Chen, J. (2018) · Nature Communications · doi:10.1038/s41467-018-04060-8 · Cited by 1,750
Self-citationAccurate Determination of Coulombic Efficiency for Lithium Metal Anodes and Lithium Metal Batteries
Adams, B. D., Zheng, J., Ren, X., Xu, W., & Zhang, J. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201702097 · Cited by 1,499
Advanced rechargeable zinc-based batteries: Recent progress and future perspectives
Li, H., Ma, L., Han, C., Wang, Z., Liu, Z., Tang, Z., & Zhi, C. (2019) · Nano Energy · doi:10.1016/j.nanoen.2019.05.059 · Cited by 1,167
Enhancing ionic conductivity in composite polymer electrolytes with well-aligned ceramic nanowires
Liu, W., Lee, S. W., Lin, D., Shi, F., Wang, S., Sendek, A. D., & Cui, Y. (2017) · Nature Energy · doi:10.1038/nenergy.2017.35 · Cited by 1,103
Zinc-ion batteries: Materials, mechanisms, and applications
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Cited by
Fundamental Concepts of Hydrogels: Synthesis, Properties, and Their Applications
Bashir, S., Hina, M., Iqbal, J., Rajpar, A. H., Mujtaba, M. A., Alghamdi, N. A., Wageh, S., Ramesh, K., & Ramesh, S. (2020) · Polymers · doi:10.3390/polym12112702 · Cited by 1,160
Huang, S., Hou, L., Li, T., Jiao, Y., & Wu, P. (2022) · Advanced Materials · doi:10.1002/adma.202110140 · Cited by 595
Wu, K., Huang, J., Yi, J., Liu, X., Liu, Y., Wang, Y., Zhang, J., & Xia, Y. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201903977 · Cited by 522
Sui, X., Guo, H., Cai, C., Li, Q., Wen, C., Zhang, X., Wang, X., Yang, J., & Zhang, L. (2021) · Chemical Engineering Journal · doi:10.1016/j.cej.2021.129478 · Cited by 445
Self-citationWang, C., Pei, Z., Meng, Q., Zhang, C., Sui, X., Yuan, Z., Wang, S., & Chen, Y. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202012030 · Cited by 394
Metadata
- Authors
- Zhu, M., Wang, X., Tang, H., Wang, J., Hao, Q., Liu, L., Li, Y., Zhang, K., & Schmidt, O. G.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2019-11-14
- Volume
- 30
- Issue
- 6
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2986137430
- Cited by
- 328
- References
- 38
- FWCI
- 13.39
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Zhu, M., Wang, X., Tang, H., Wang, J., Hao, Q., Liu, L., Li, Y., Zhang, K., & Schmidt, O. G. (2020). Antifreezing Hydrogel with High Zinc Reversibility for Flexible and Durable Aqueous Batteries by Cooperative Hydrated Cations. Advanced Functional Materials. https://doi.org/10.1002/adfm.201907218
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