The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Accurate Determination of Coulombic Efficiency for Lithium Metal Anodes and Lithium Metal Batteries
Abstract
Lithium (Li) metal is an ideal anode material for high energy density batteries. However, the low Coulombic efficiency (CE) and the formation of dendrites during repeated plating and stripping processes have hindered its applications in rechargeable Li metal batteries. The accurate measurement of Li CE is a critical factor to predict the cycle life of Li metal batteries, but the measurement of Li CE is affected by various factors that often lead to conflicting values reported in the literature. Here, several parameters that affect the measurement of Li CE are investigated and a more accurate method of determining Li CE is proposed. It is also found that the capacity used for cycling greatly affects the stabilization cycles and the average CE. A higher cycling capacity leads to faster stabilization of Li anode and a higher average CE. With a proper operating protocol, the average Li CE can be increased from 99.0% to 99.5% at a high capacity of 6 mA h cm−2 (which is suitable for practical applications) when a high‐concentration ether‐based electrolyte is used.
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Citations
Cites
Reviving the lithium metal anode for high-energy batteries
Lin, D., Liu, Y., & Cui, Y. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2017.16 · Cited by 6,763
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
High rate and stable cycling of lithium metal anode
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Self-citationAdvanced Model for Solid Electrolyte Interphase Electrodes in Liquid and Polymer Electrolytes
Peled, E., Golodnitsky, D., & Ardel, G. (1997) · Journal of The Electrochemical Society · doi:10.1149/1.1837858 · Cited by 1,205
The Surface Chemistry of Lithium Electrodes in Alkyl Carbonate Solutions
Aurbach, D., Ein‐Ely, Y., & Zaban, A. (1994) · Journal of The Electrochemical Society · doi:10.1149/1.2054718 · Cited by 344
Cited by
Pathways for practical high-energy long-cycling lithium metal batteries
Liu, J., Bao, Z., Cui, Y., Dufek, E. J., Goodenough, J. B., Khalifah, P., Li, Q., Liaw, B. Y., Liu, P., Manthiram, A., et al. (2019) · Nature Energy · doi:10.1038/s41560-019-0338-x · Cited by 3,412
Self-citationTailoring electrolyte solvation for Li metal batteries cycled at ultra-low temperature
Holoubek, J., Liu, H., Wu, Z., Yin, Y., Xing, X., Cai, G., Yu, S., Zhou, H., Pascal, T. A., Chen, Z., et al. (2021) · Nature Energy · doi:10.1038/s41560-021-00783-z · Cited by 851
High-Efficiency Lithium Metal Batteries with Fire-Retardant Electrolytes
Chen, S., Zheng, J., Yu, L., Ren, X., Engelhard, M. H., Niu, C., Lee, H., Xu, W., Xiao, J., Liu, J., et al. (2018) · Joule · doi:10.1016/j.joule.2018.05.002 · Cited by 654
Self-citationRecent developments and insights into the understanding of Na metal anodes for Na-metal batteries
Zhao, Y., Adair, K. R., & Sun, X. (2018) · Energy & Environmental Science · doi:10.1039/c8ee01373j · Cited by 533
Li, Y., Huang, W., Li, Y., Pei, A., Boyle, D. T., & Cui, Y. (2018) · Joule · doi:10.1016/j.joule.2018.08.004 · Cited by 459
Metadata
- Authors
- Adams, B. D., Zheng, J., Ren, X., Xu, W., & Zhang, J.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2017-10-11
- Volume
- 8
- Issue
- 7
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2763902109
- Cited by
- 1,499
- References
- 5
- FWCI
- 20.14
- Type
- journal article
- Language
- en
- Open access
- closed
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