The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
High‐Power Lithium Metal Batteries Enabled by High‐Concentration Acetonitrile‐Based Electrolytes with Vinylene Carbonate Additive
Abstract
To enable next‐generation high‐power, high‐energy‐density lithium (Li) metal batteries (LMBs), an electrolyte possessing both high Li Coulombic efficiency (CE) at a high rate and good anodic stability on cathodes is critical. Acetonitrile (AN) is a well‐known organic solvent for high anodic stability and high ionic conductivity, yet its application in LMBs is limited due to its poor compatibility with Li metal anodes even at high salt concentration conditions. Here, a highly concentrated AN‐based electrolyte is developed with a vinylene carbonate (VC) additive to suppress Li+ depletion at high current densities. Addition of VC to the AN‐based electrolyte leads to the formation of a polycarbonate‐based solid electrolyte interphase, which minimizes Li corrosion and leads to a very high Li CE of up to 99.2% at a current density of 0.2 mA cm‐2. Using such an electrolyte, fast charging of Li||NMC333 cells is realized at a high current density of 3.6 mA cm‐2, and stable cycling of Li||NMC622 cells with a high cathode loading of 4 mAh cm‐2 is also demonstrated.
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Cites
High rate and stable cycling of lithium metal anode
Qian, J., Henderson, W. A., Xu, W., Bhattacharya, P., Engelhard, M., Borodin, O., & Zhang, J.-G. (2015) · Nature Communications · doi:10.1038/ncomms7362 · Cited by 2,561
Self-citationFluoroethylene Carbonate Additives to Render Uniform Li Deposits in Lithium Metal Batteries
Zhang, X., Cheng, X., Chen, X., Yan, C., & Zhang, Q. (2017) · Advanced Functional Materials · doi:10.1002/adfm.201605989 · Cited by 1,699
Safe and high-rate supercapacitors based on an “acetonitrile/water in salt” hybrid electrolyte
Dou, Q., Lei, S., Wang, D.-W., Zhang, Q., Xiao, D., Guo, H., Wang, A., Yang, H., Li, Y., Shi, S., et al. (2018) · Energy & Environmental Science · doi:10.1039/c8ee01040d · Cited by 435
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Cited by
Fast charging of energy-dense lithium-ion batteries
Wang, C.-Y., Liu, T., Yang, X.-G., Ge, S., Stanley, N. V., Rountree, E. S., Leng, Y., & McCarthy, B. D. (2022) · Nature · doi:10.1038/s41586-022-05281-0 · Cited by 988
Emerging Era of Electrolyte Solvation Structure and Interfacial Model in Batteries
Cheng, H., Sun, Q., Li, L., Zou, Y., Wang, Y., Cai, T., Zhao, F., Liu, G., Ma, Z., Wahyudi, W., et al. (2022) · ACS Energy Letters · doi:10.1021/acsenergylett.1c02425 · Cited by 640
Self-citationA Review of Solid Electrolyte Interphase (SEI) and Dendrite Formation in Lithium Batteries
Li, B., Chao, Y., Li, M., Xiao, Y., Li, R., Yang, K., Cui, X., Xu, G., Li, L., Yang, C., et al. (2023) · Electrochemical Energy Reviews · doi:10.1007/s41918-022-00147-5 · Cited by 406
Self-citationCritical effects of electrolyte recipes for Li and Na metal batteries
Zheng, X., Huang, L., Ye, X., Zhang, J., Min, F., Luo, W., & Huang, Y. (2021) · Chem · doi:10.1016/j.chempr.2021.02.025 · Cited by 367
Self-citationCao, Z., Zheng, X., Qu, Q., Huang, Y., & Zheng, H. (2021) · Advanced Materials · doi:10.1002/adma.202103178 · Cited by 336
Metadata
- Authors
- Peng, Z., Cao, X., Gao, P., Jia, H., Ren, X., Roy, S., Li, Z., Zhu, Y., Xie, W., Liu, D., Li, Q., Wang, D., Xu, W., & Zhang, J.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2020-04-27
- Volume
- 30
- Issue
- 24
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W3017712197
- Cited by
- 217
- References
- 3
- FWCI
- 9.79
- Type
- journal article
- Language
- en
- Open access
- closed
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- Peng, Z., Cao, X., Gao, P., Jia, H., Ren, X., Roy, S., Li, Z., Zhu, Y., Xie, W., Liu, D., Li, Q., Wang, D., Xu, W., & Zhang, J. (2020). High‐Power Lithium Metal Batteries Enabled by High‐Concentration Acetonitrile‐Based Electrolytes with Vinylene Carbonate Additive. Advanced Functional Materials. https://doi.org/10.1002/adfm.202001285
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