The DOI matches its Crossref record; 145 of the 145 references it cites were found in a registry or an index.
Challenges and Strategies to Advance High‐Energy Nickel‐Rich Layered Lithium Transition Metal Oxide Cathodes for Harsh Operation
Abstract
Nickel‐rich layered lithium transition metal oxides (LiNi 1−x−yCoxMnyO 2 and LiNi 1−x−yCoxAlyO 2, x + y ≤ 0.2) are the most attractive cathode materials for the next generation lithium‐ion batteries for automotive application. However, they suffer from structural/interfacial instability during repeated charge/discharge, resulting in severe performance degradation and serious safety concerns. This work provides a comprehensive review about challenges and strategies to advance nickel‐rich layered cathodes specifically for harsh (high‐voltage, high‐temperature, and fast charging) operations. Firstly, the degradation pathways of nickel‐rich cathodes including surface/interface degradation, undesired cathode–electrolytes parasitic reactions, gas evolution, inter/intragranular cracking, and electrical/ionic isolation are discussed. Then, recent achievements in stabilizing the structure/interface of nickel‐rich cathodes via surface coating, cation/anion doping, composition tailoring, morphology engineering, and electrolytes optimization are summarized. Moreover, challenges and strategies to improve the performance of Ni‐rich cathodes at the electrode level are discussed. Outlook and perspectives to promote the practical application of nickel‐rich layered cathodes toward automotive application are provided as well.
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Cites
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
Pathways for practical high-energy long-cycling lithium metal batteries
Liu, J., Bao, Z., Cui, Y., Dufek, E. J., Goodenough, J. B., Khalifah, P., Li, Q., Liaw, B. Y., Liu, P., Manthiram, A., et al. (2019) · Nature Energy · doi:10.1038/s41560-019-0338-x · Cited by 3,412
Performance and cost of materials for lithium-based rechargeable automotive batteries
Schmuch, R., Wagner, R., Hörpel, G., Placke, T., & Winter, M. (2018) · Nature Energy · doi:10.1038/s41560-018-0107-2 · Cited by 3,233
Batteries and fuel cells for emerging electric vehicle markets
Cano, Z. P., Banham, D., Ye, S., Hintennach, A., Lu, J., Fowler, M., & Chen, Z. (2018) · Nature Energy · doi:10.1038/s41560-018-0108-1 · Cited by 2,873
Self-citationNoh, H.-J., Youn, S., Yoon, C. S., & Sun, Y.-K. (2013) · Journal of Power Sources · doi:10.1016/j.jpowsour.2013.01.063 · Cited by 2,302
Aurbach, D. (2000) · Journal of Power Sources · doi:10.1016/s0378-7753(00)00431-6 · Cited by 2,130
Nickel‐Rich Layered Lithium Transition‐Metal Oxide for High‐Energy Lithium‐Ion Batteries
Liu, W., Oh, P., Liu, X., Lee, M., Cho, W., Chae, S., Kim, Y., & Cho, J. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201409262 · Cited by 1,960
Self-citationHigh-nickel layered oxide cathodes for lithium-based automotive batteries
Li, W., Erickson, E. M., & Manthiram, A. (2020) · Nature Energy · doi:10.1038/s41560-019-0513-0 · Cited by 1,754
Ryu, H.-H., Park, K.-J., Yoon, C. S., & Sun, Y.-K. (2018) · Chemistry of Materials · doi:10.1021/acs.chemmater.7b05269 · Cited by 1,629
Commercialization of Lithium Battery Technologies for Electric Vehicles
Zeng, X., Li, M., Abd El‐Hady, D., Alshitari, W., Al‐Bogami, A. S., Lu, J., & Amine, K. (2019) · Advanced Energy Materials · doi:10.1002/aenm.201900161 · Cited by 1,542
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Cited by
Mechanical properties of cathode materials for lithium-ion batteries
Stallard, J. C., Wheatcroft, L., Booth, S. G., Boston, R., Corr, S. A., De Volder, M. F. L., Inkson, B. J., & Fleck, N. A. (2022) · Joule · doi:10.1016/j.joule.2022.04.001 · Cited by 336
Wang, J., Li, D., Zeng, W., Chen, X., Zhang, Y., Zhang, S., Li, Z., Li, C., & Mu, S. (2025) · Journal of Energy Chemistry · doi:10.1016/j.jechem.2024.11.016 · Cited by 62
Metadata
- Authors
- Xu, G., Liu, X., Daali, A., Amine, R., Chen, Z., & Amine, K.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2020-09-09
- Volume
- 30
- Issue
- 46
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W3084230050
- Cited by
- 313
- References
- 145
- FWCI
- 11.82
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xu, G., Liu, X., Daali, A., Amine, R., Chen, Z., & Amine, K. (2020). Challenges and Strategies to Advance High‐Energy Nickel‐Rich Layered Lithium Transition Metal Oxide Cathodes for Harsh Operation. Advanced Functional Materials. https://doi.org/10.1002/adfm.202004748
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