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An Overall Reaction Integrated with Highly Selective Oxidation of 5‐Hydroxymethylfurfural and Efficient Hydrogen Evolution
Open accessAbstract
Thermodynamically favorable electrooxidation reactions of biomass derivatives integrated with hydrogen evolution reaction (HER) can simultaneously provide value‐added chemicals and hydrogen, and eventually meeting the need for clean and sustainable energy development. Herein, the integration of a six‐electron involved anodic half‐reaction‐selective electrooxidation of 5‐hydroxymethylfurfural into 2,5‐furandicarboxylic acid (FDCA) on a hierarchically layered double hydroxide (CoFe@NiFe) with a cathodic HER in a two‐chamber system is reported. The overall reaction reaches 38 mA cm−2 at 1.40 V and exhibits 100% selectivity to yield FDCA and a nearly 100% Faraday efficiency with hydrogen production of 901 µmol cm−2. Several operando techniques confirm that the trivalent nickel species in the CoFe@NiFe catalyst are mainly responsible for this 100%‐selective oxidation reaction. This integrated overall reaction is thus a new strategy to utilize cheap catalysts and biomass derivatives to simultaneously produce value‐added chemicals and sustainable energy materials, and eventually to solve current challenges of energy depletion and environmental pollution.
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Design of electrocatalysts for oxygen- and hydrogen-involving energy conversion reactions
Jiao, Y., Zheng, Y., Jaroniec, M., & Qiao, S. Z. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00470a · Cited by 5,388
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Computational high-throughput screening of electrocatalytic materials for hydrogen evolution
Greeley, J., Jaramillo, T. F., Bonde, J., Chorkendorff, I., & Nørskov, J. K. (2006) · Nature Materials · doi:10.1038/nmat1752 · Cited by 4,097
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Toward the rational design of non-precious transition metal oxides for oxygen electrocatalysis
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Replacing fossil based PET with biobased PEF; process analysis, energy and GHG balance
Eerhart, A. J. J. E., Faaij, A. P. C., & Patel, M. K. (2012) · Energy & Environmental Science · doi:10.1039/c2ee02480b · Cited by 666
Cited by
Shih, A. J., Monteiro, M. C. O., Dattila, F., Pavesi, D., Philips, M., da Silva, A. H. M., Vos, R. E., Ojha, K., Park, S., van der Heijden, O., et al. (2022) · Nature Reviews Methods Primers · doi:10.1038/s43586-022-00164-0 · Cited by 521
Zhao, H., Yue, Y., Fan, Y., Wang, J., Li, W., Wei, F., Liu, M., Yu, Y., Lu, W., & Zhang, G. (2022) · ChemSusChem · doi:10.1002/cssc.202201625 · Cited by 27
Metadata
- Authors
- Xie, Y., Zhou, Z., Yang, N., & Zhao, G.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2021-05-18
- Volume
- 31
- Issue
- 34
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W3162429781
- Cited by
- 173
- References
- 6
- FWCI
- 8.96
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Xie, Y., Zhou, Z., Yang, N., & Zhao, G. (2021). An Overall Reaction Integrated with Highly Selective Oxidation of 5‐Hydroxymethylfurfural and Efficient Hydrogen Evolution. Advanced Functional Materials. https://doi.org/10.1002/adfm.202102886
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