The DOI matches its Crossref record; 38 of the 38 references it cites were found in a registry or an index.
Synergistic Solvation and Interface Regulations of Eco‐Friendly Silk Peptide Additive Enabling Stable Aqueous Zinc‐Ion Batteries
Abstract
Aqueous Zn‐ion batteries have aroused much attention recently, yet challenges still exist in the lack of low‐cost, highly stable electrolytes to tackle the serious side reactions at Zn anode–electrolyte interface. Herein, a ZnSO 4‐based low‐cost aqueous electrolyte is demonstrated with a small amount of eco‐friendly silk peptide as an efficient additive. Compared with silk sericin and fibroin, silk peptide with abundant strong polar groups (COOH and NH 2) suppresses the side reactions. Namely, silk peptide regulates the solvation structure of Zn 2+ to decrease coordinated active H 2 O and SO 42−, and tends to anchor on Zn anode surface for the isolation of contact H 2 O/SO 42− as well as electrostatic shielding, demonstrating synergistic solvation and interface regulating effect. Consequently, the excellent cycle life (3000 h) and Coulombic efficiency (99.7%) of Zn anodes are revealed in 2 m ZnSO 4 electrolyte with only 5 mg mL−1 of silk peptide (≈0.49 USD L−1), promising practical applications of reversible zinc‐ion batteries.
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Cites
Infrared spectroscopy of proteins
Barth, A. (2007) · Biochimica et Biophysica Acta (BBA) - Bioenergetics · doi:10.1016/j.bbabio.2007.06.004 · Cited by 5,129
Highly reversible zinc metal anode for aqueous batteries
Wang, F., Borodin, O., Gao, T., Fan, X., Sun, W., Han, F., Faraone, A., Dura, J. A., Xu, K., & Wang, C. (2018) · Nature Materials · doi:10.1038/s41563-018-0063-z · Cited by 3,305
Materials fabrication from Bombyx mori silk fibroin
Rockwood, D. N., Preda, R. C., Yücel, T., Wang, X., Lovett, M. L., & Kaplan, D. L. (2011) · Nature Protocols · doi:10.1038/nprot.2011.379 · Cited by 3,066
Recent Advances in Aqueous Zinc-Ion Batteries
Fang, G., Zhou, J., Pan, A., & Liang, S. (2018) · ACS Energy Letters · doi:10.1021/acsenergylett.8b01426 · Cited by 2,258
Recent Advances in Zn‐Ion Batteries
Song, M., Tan, H., Chao, D., & Fan, H. J. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201802564 · Cited by 2,196
Scientific Challenges for the Implementation of Zn-Ion Batteries
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Dendrite-Free Lithium Deposition via Self-Healing Electrostatic Shield Mechanism
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Roadmap for advanced aqueous batteries: From design of materials to applications
Chao, D., Zhou, W., Xie, F., Ye, C., Li, H., Jaroniec, M., & Qiao, S.-Z. (2020) · Science Advances · doi:10.1126/sciadv.aba4098 · Cited by 1,940
Reversible epitaxial electrodeposition of metals in battery anodes
Zheng, J., Zhao, Q., Tang, T., Yin, J., Quilty, C. D., Renderos, G. D., Liu, X., Deng, Y., Wang, L., Bock, D. C., et al. (2019) · Science · doi:10.1126/science.aax6873 · Cited by 1,877
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Metadata
- Authors
- Wang, B., Zheng, R., Yang, W., Han, X., Hou, C., Zhang, Q., Li, Y., Li, K., & Wang, H.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2022-03-03
- Volume
- 32
- Issue
- 23
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W4214946890
- Cited by
- 257
- References
- 38
- FWCI
- 15.79
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, B., Zheng, R., Yang, W., Han, X., Hou, C., Zhang, Q., Li, Y., Li, K., & Wang, H. (2022). Synergistic Solvation and Interface Regulations of Eco‐Friendly Silk Peptide Additive Enabling Stable Aqueous Zinc‐Ion Batteries. Advanced Functional Materials. https://doi.org/10.1002/adfm.202112693
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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