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Triple Interface Optimization of Ru‐based Electrocatalyst with Enhanced Activity and Stability for Hydrogen Evolution Reaction
Open accessAbstract
A challenging task is to promote Ru atom economy and simultaneously alleviate Ru dissolution during the hydrogen evolution reaction (HER) process. Herein, Ru nanograins (≈1.7 nm in size) uniformly grown on 1 T‐MoS 2 lace‐decorated Ti 3 C 2 T x MXene sheets (Ru@1 T‐MoS 2‐MXene) are successfully synthesized with three types of interfaces (Ru/MoS 2, Ru/MXene, and MoS 2/MXene). It gives high mass activity of 0.79 mA µg Ru−1 at an overpotential of 100 mV, which is ≈36 times that of Ru NPs. It also has a much smaller Ru dissolution rate (9 ng h−1), accounting for 22% of the rate for Ru NPs. Electrochemical tests, scanning electrochemical microscopy measurements combined with DFT calculations disclose the role of triple interface optimization in improved activity and stability. First, 2D MoS 2 and MXene can well disperse and stabilize Ru grains, giving larger electrochemical active area. Then, Ru/MoS 2 interfaces weakening H* adsorption energy and Ru/MXene interfaces enhancing electrical conductivity, can efficiently improve the activity. Next, MoS 2/MXene interfaces can protect MXene sheet edges from oxidation and keep 1 T‐MoS 2 phase stability during the long‐term catalytic process. Meanwhile, Ru@1 T‐MoS 2‐MXene also displays superior activity and stability in neutral and alkaline media. This work provides a multiple‐interface optimization route to develop high‐efficiency and durable pH‐universal Ru‐based HER electrocatalysts.
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Metadata
- Authors
- Li, G., Sun, T., Niu, H., Yan, Y., Liu, T., Jiang, S., Yang, Q., Zhou, W., & Guo, L.
- Affiliations
- School of Chemistry Beijing Advanced Innovation Center for Biomedical Engineering Beihang University Beijing 100191 China
- Qingdao University (CN)
- Beihang University (CN)
- Corresponding author
- Zhou, Wei
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2023-01-17
- Volume
- 33
- Issue
- 13
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W4319836484
- Semantic Scholar
- ff44520d83108513c4b22d6cf80c6b055d4edca9
- Cited by
- 130
- References
- 63
- Citations by year
- 2026: 18 · 2025: 41 · 2024: 46 · 2023: 25
- FWCI
- 6.20
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Locations
- Advanced Functional Materials (publishedVersion)
- Funders
- National Natural Science Foundation of China (52172176, 51972011)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Physical Sciences › Materials Science › Materials Chemistry › Hydrogen Storage and Materials
- Keywords
- hydrogen evolution reaction, ruthenium electrocatalysts, 1T-MoS2, MXene, Ti3C2Tx, H* adsorption energy, edge protection, pH-universal catalysis, alkaline electrocatalysis, mass activity
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