A Hybrid Photocatalytic System Splits Atmospheric Water to Produce Hydrogen
Open accessAbstract
Large‐scale photocatalytic water‐splitting panel reactor system is developed and demonstrated its commercial feasibility. However, water scarcity is one of the leading challenges for the sustainable development of photocatalytic hydrogen generation in a well‐lit area. Here, a water harvesting form air‐photothermal water evaporation‐photocatalytic hydrogen evolution (AWPH) system is devised. The hybrid system comprising carbonized wood (CWx) combined with the hygroscopic salt ZnCl 2 and Pt‐modified g‐C 3 N 4 nanosheets (Pt‐CN) as a photocatalyst is developed, in which the carbonized wood has a vertical pore structure that can provide attachment sites for the hygroscopic salt. The water adsorbed by ZnCl 2 is driven along the vertical pore channels to the photocatalyst due to the photothermal conversion effect. The bi‐phase interfaces of vapor/photocatalyst/hydrogen produced by the photothermal‐photocatalytic system significantly reduce the interface barrier and substantially lower the resistance to hydrogen transport. CW550 exhibited a water uptake of 0.56 g g−1 and hydrogen yield of 21.99 µmol cm−2 under 100 mW cm−2 illumination at a flow rate of 2 mL min−1 for 5 h and a half at atmospheric pressure.
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The performance surpasses previously reported aerogel-based platforms, including directional pore-structured carbonized wood (39.98 mmol m−2 h−1) and photothermal-photocatalytic layered aerogels (17.94 mmol m−2 h−1).
“Additionally, the performance surpasses that of previously reported aerogel-based platforms, including the photocatalytic system consisting of directional pore-structured carbonized wood (39.98 mmol m 2 h 1 ) 64 and photothermalphotocatalytic layered aerogels (17.94 mmol m 2 h 1 ), 65 although it remains slightly lower than the most recent advanced designs (163 mmol m 2 h 1 ). 63”
From Gradient-structured directional porous floatable aerogels for effective solar-driven hydrogen production and steam generation (2025) · cites this paper as [64]
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- Authors
- He, L., Zeng, X., Chen, H., Zhao, L., Huang, Z., Wang, D., He, X., Fang, W., Du, X., & Li, W.
- Affiliations
- Wuhan University of Science and Technology (CN)
- Hunan University (CN)
- Corresponding author
- Chen, Hui
- Zhao, Lei
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2024-01-09
- Volume
- 34
- Issue
- 19
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W4390698259
- Cited by
- 56
- References
- 56
- Citations by year
- 2026: 12 · 2025: 31 · 2024: 13
- FWCI
- 3.73
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Locations
- Advanced Functional Materials (publishedVersion)
- Funders
- National Natural Science Foundation of China (22105151)
- Natural Science Foundation of Hubei Province (2021CFB469, 2021CFB124, 2022CFB626)
- Wuhan University of Science and Technology (2023A0305)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Solar-Powered Water Purification Methods
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › TiO2 Photocatalysis and Solar Cells
- Keywords
- photocatalytic hydrogen evolution, atmospheric water harvesting, photothermal evaporation, carbonized wood, water adsorption
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