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Dynamically Restructuring Hydrogel Networks Formed with Reversible Covalent Crosslinks
Abstract
Dynamically restructuring hydrogel networks are formed from two water-soluble polymers by functionalization with phenylboronic acid (PBA) and salicylhydroxamic acid (SHA) moieties that interact through pH-sensitive and reversible covalent crosslinks (see figure). The networks can be tuned to display a wide range of pH-responsive properties, which can potentially be exploited for drug delivery systems in biological environments where similar acidic changes occur.
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Cited by
Holten-Andersen, N., Harrington, M. J., Birkedal, H., Lee, B. P., Messersmith, P. B., Lee, K. Y. C., & Waite, J. H. (2011) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1015862108 · Cited by 1,597
Soft Materials by Design: Unconventional Polymer Networks Give Extreme Properties
Zhao, X., Chen, X., Yuk, H., Lin, S., Liu, X., & Parada, G. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c01088 · Cited by 1,161
Self-healing gels based on constitutional dynamic chemistry and their potential applications
Wei, Z., Yang, J. H., Zhou, J., Xu, F., Zrínyi, M., Dussault, P. H., Osada, Y., & Chen, Y. M. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00219a · Cited by 896
The design of reversible hydrogels to capture extracellular matrix dynamics
Rosales, A. M., & Anseth, K. S. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2015.12 · Cited by 772
Vitrimers: Permanently crosslinked polymers with dynamic network topology
Van Zee, N. J., & Nicolaÿ, R. (2020) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2020.101233 · Cited by 734
Metadata
- Authors
- Roberts, M. C., Hanson, M. C., Massey, A. P., Karren, E. A., & Kiser, P. F.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2007-08-09
- Volume
- 19
- Issue
- 18
- Pages
- 2503-2507
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2164542218
- Cited by
- 236
- References
- 0
- FWCI
- 1.76
- Type
- journal article
- Language
- en
- Open access
- closed
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- Roberts, M. C., Hanson, M. C., Massey, A. P., Karren, E. A., & Kiser, P. F. (2007). Dynamically Restructuring Hydrogel Networks Formed with Reversible Covalent Crosslinks. Advanced Materials. https://doi.org/10.1002/adma.200602649
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
