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Alkali‐Assisted Synthesis of Nitrogen Deficient Graphitic Carbon Nitride with Tunable Band Structures for Efficient Visible‐Light‐Driven Hydrogen Evolution
Abstract
A facile synthetic strategy for nitrogen-deficient graphitic carbon nitride (g-C3Nx) is established, involving a simple alkali-assisted thermal polymerization of urea, melamine, or thiourea. In situ introduced nitrogen vacancies significantly redshift the absorption edge of g-C3Nx, with the defect concentration depending on the alkali to nitrogen precursor ratio. The g-C3Nx products show superior visible-light photocatalytic performance compared to pristine g-C3N4.
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Cites
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
Cui, Y., Ding, Z., Liu, P., Antonietti, M., Fu, X., & Wang, X. (2012) · Phys. Chem. Chem. Phys. · doi:10.1039/c1cp22820j · Cited by 585
Cited by
Ren, Y., Zeng, D., & Ong, W.-J. (2019) · Chinese Journal of Catalysis · doi:10.1016/s1872-2067(19)63293-6 · Cited by 528
Surface Modification of 2D Photocatalysts for Solar Energy Conversion
Feng, C., Wu, Z., Huang, K., Ye, J., & Zhang, H. (2022) · Advanced Materials · doi:10.1002/adma.202200180 · Cited by 456
Yang, M., Gao, M., Hong, M., & Ho, G. W. (2018) · Advanced Materials · doi:10.1002/adma.201802894 · Cited by 389
Xia, P., Antonietti, M., Zhu, B., Heil, T., Yu, J., & Cao, S. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201900093 · Cited by 367
Yang, X., Tian, L., Zhao, X., Tang, H., Liu, Q., & Li, G. (2019) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2018.11.056 · Cited by 348
Metadata
- Authors
- Yu, H., Shi, R., Zhao, Y., Bian, T., Zhao, Y., Zhou, C., Waterhouse, G. I. N., Wu, L., Tung, C., & Zhang, T.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-02-10
- Volume
- 29
- Issue
- 16
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2587681799
- Cited by
- 2,257
- References
- 2
- FWCI
- 53.08
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yu, H., Shi, R., Zhao, Y., Bian, T., Zhao, Y., Zhou, C., Waterhouse, G. I. N., Wu, L., Tung, C., & Zhang, T. (2017). Alkali‐Assisted Synthesis of Nitrogen Deficient Graphitic Carbon Nitride with Tunable Band Structures for Efficient Visible‐Light‐Driven Hydrogen Evolution. Advanced Materials. https://doi.org/10.1002/adma.201605148
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