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Cited by 456Advanced Photocatalysis Techniques2D Materials and ApplicationsTiO2 Photocatalysis and Solar Cells

Surface Modification of 2D Photocatalysts for Solar Energy Conversion

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Feng, Chengyang, Wu, Zhi‐Peng, Huang, Kuo‐Wei, Ye, Jinhua, Zhang, Huabin·2022·Advanced Materials
DOI 10.1002/adma.202200180
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Abstract

2D materials show many particular properties, such as high surface‐to‐volume ratio, high anisotropic degree, and adjustable chemical functionality. These unique properties in 2D materials have sparked immense interest due to their applications in photocatalytic systems, resulting in significantly enhanced light capture, charge‐transfer kinetics, and surface reaction. Herein, the research progress in 2D photocatalysts based on varied compositions and functions, followed by specific surface modification strategies, is introduced. Fundamental principles focusing on light harvesting, charge separation, and molecular adsorption/activation in the 2D‐material‐based photocatalytic system are systemically explored. The examples described here detail the use of 2D materials in various photocatalytic energy‐conversion systems, including water splitting, carbon dioxide reduction, nitrogen fixation, hydrogen peroxide production, and organic synthesis. Finally, by elaborating the challenges and possible solutions for developing these 2D materials, the review is expected to provide some inspiration for the future research of 2D materials used on efficient photocatalytic energy conversions.

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  • The low electronic conductivity, wide band gap, rapid charge carrier recombination, and small accessible surface active sites of carbon nitride greatly limit its application in water splitting and photosynthesis.

    “Unfortunately, the low electronic conductivity, wide band gap, rapid charge carrier recombination behavior, as well as the fairly small accessible surface active sites, have greatly limited its application in water splitting and photosynthesis [6, 7].”

    From Unveiling N-doped carbon nitride aerogel for efficient electrocatalytic water splitting application (2025) · cites this paper as [7]

    Section 2.1.1 says limited surface exposure severely inhibits the catalytic activity of bulk graphitic carbon nitride. The paper also reports that carbon vacancies inhibit charge recombination and improve hydrogen production, supporting that limitation. But §2.1.1 calls its 2.7 eV band gap “narrow,” not wide; the cited passages do not establish low electronic conductivity or a limitation specific to photosynthesis. (LLM, conf=0.86)

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Cited by

Sorted by citations

Authors
Feng, C., Wu, Z., Huang, K., Ye, J., & Zhang, H.
Affiliations
  • King Abdullah University of Science and Technology (SA)
  • National Institute for Materials Science (JP)
ORCID
Venue
Advanced Materials
Publisher
Wiley
Published
2022-04-03
Volume
34
Issue
23
Pages
e2200180-e2200180
ISSN
  • 0935-9648 (ISSN-L)
  • 1521-4095
DOI
10.1002/adma.202200180
OpenAlex
W4221059889
Cited by
456
References
1
Citations by year
2026: 53 · 2025: 107 · 2024: 133 · 2023: 108 · 2022: 55
FWCI
6.39
Type
journal article
Language
en
Open access
Licence
Locations
  • Advanced Materials (publishedVersion, cc-by)
  • PubMed (publishedVersion)
  • King Abdullah University of Science and Technology Repository (King Abdullah University of Science and Technology) (submittedVersion)
Funders
King Abdullah University of Science and Technology
Topics
  • Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
  • Physical Sciences › Materials Science › Materials Chemistry › 2D Materials and Applications
  • Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › TiO2 Photocatalysis and Solar Cells
Keywords
two-dimensional materials, surface modification, photocatalysis, solar energy conversion, light harvesting, charge separation, molecular adsorption, water splitting, carbon dioxide reduction, nitrogen fixation, hydrogen peroxide production, photocatalytic organic synthesis

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