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Tri‐s‐triazine‐Based Crystalline Carbon Nitride Nanosheets for an Improved Hydrogen Evolution
Abstract
Tri‐s‐triazine‐based crystalline carbon nitride nanosheets (CCNNSs) have been successfully extracted via a conventional and cost‐effective sonication–centrifugation process. These CCNNSs possess a highly defined and unambiguous structure with minimal thickness, large aspect ratios, homogeneous tri‐s‐triazine‐based units, and high crystallinity. These tri‐s‐triazine‐based CCNNSs show significantly enhanced photocatalytic hydrogen generation activity under visible light than g‐C 3 N 4, poly (triazine imide)/Li+ Cl–, and bulk tri‐s‐triazine‐based crystalline carbon nitrides. A highly apparent quantum efficiency of 8.57% at 420 nm for hydrogen production from aqueous methanol feedstock can be achieved from tri‐s‐triazine‐based CCNNSs, exceeding most of the reported carbon nitride nanosheets. Benefiting from the inherent structure of 2D crystals, the ultrathin tri‐s‐triazine‐based CCNNSs provide a broad range of application prospects in the fields of bioimaging, and energy storage and conversion.
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Citations
Cites
Selective Breaking of Hydrogen Bonds of Layered Carbon Nitride for Visible Light Photocatalysis
Kang, Y., Yang, Y., Yin, L., Kang, X., Wang, L., Liu, G., & Cheng, H. (2016) · Advanced Materials · doi:10.1002/adma.201601567 · Cited by 626
Cited by
Tan, M., Ma, Y., Yu, C., Luan, Q., Li, J., Liu, C., Dong, W., Su, Y., Qiao, L., Gao, L., et al. (2022) · Advanced Functional Materials · doi:10.1002/adfm.202111740 · Cited by 394
Xia, P., Antonietti, M., Zhu, B., Heil, T., Yu, J., & Cao, S. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201900093 · Cited by 367
Xu, G., Zhang, H., Wei, J., Zhang, H.-X., Wu, X., Li, Y., Li, C., Zhang, J., & Ye, J. (2018) · ACS Nano · doi:10.1021/acsnano.8b00110 · Cited by 298
Wang, Q., Zhao, Z. L., Dong, S., He, D., Lawrence, M. J., Han, S., Cai, C., Xiang, S., Rodriguez, P., Xiang, B., et al. (2018) · Nano Energy · doi:10.1016/j.nanoen.2018.09.003 · Cited by 273
Metadata
- Authors
- Ou, H., Lin, L., Zheng, Y., Yang, P., Fang, Y., & Wang, X.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-04-12
- Volume
- 29
- Issue
- 22
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2605927619
- Cited by
- 675
- References
- 1
- FWCI
- 21.13
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ou, H., Lin, L., Zheng, Y., Yang, P., Fang, Y., & Wang, X. (2017). Tri‐s‐triazine‐Based Crystalline Carbon Nitride Nanosheets for an Improved Hydrogen Evolution. Advanced Materials. https://doi.org/10.1002/adma.201700008
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