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Peapod‐like Li3VO4/N‐Doped Carbon Nanowires with Pseudocapacitive Properties as Advanced Materials for High‐Energy Lithium‐Ion Capacitors
Abstract
Lithium ion capacitors are new energy storage devices combining the complementary features of both electric double‐layer capacitors and lithium ion batteries. A key limitation to this technology is the kinetic imbalance between the Faradaic insertion electrode and capacitive electrode. Here, we demonstrate that the Li 3 VO 4 with low Li‐ion insertion voltage and fast kinetics can be favorably used for lithium ion capacitors. N‐doped carbon‐encapsulated Li 3 VO 4 nanowires are synthesized through a morphology‐inheritance route, displaying a low insertion voltage between 0.2 and 1.0 V, a high reversible capacity of ≈400 mAh g−1 at 0.1 A g−1, excellent rate capability, and long‐term cycling stability. Benefiting from the small nanoparticles, low energy diffusion barrier and highly localized charge‐transfer, the Li 3 VO 4/N‐doped carbon nanowires exhibit a high‐rate pseudocapacitive behavior. A lithium ion capacitor device based on these Li 3 VO 4/N‐doped carbon nanowires delivers a high energy density of 136.4 Wh kg−1 at a power density of 532 W kg−1, revealing the potential for application in high‐performance and long life energy storage devices.
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Cites
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Supercapacitors as next generation energy storage devices: Properties and applications
Olabi, A. G., Abbas, Q., Al Makky, A., & Abdelkareem, M. A. (2022) · Energy · doi:10.1016/j.energy.2022.123617 · Cited by 960
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Metadata
- Authors
- Shen, L., Lv, H., Chen, S., Kopold, P., van Aken, P. A., Wu, X., Maier, J., & Yu, Y.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-05-03
- Volume
- 29
- Issue
- 27
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2611891973
- Cited by
- 382
- References
- 40
- FWCI
- 16.46
- Type
- journal article
- Language
- en
- Open access
- closed
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- Shen, L., Lv, H., Chen, S., Kopold, P., van Aken, P. A., Wu, X., Maier, J., & Yu, Y. (2017). Peapod‐like Li3VO4/N‐Doped Carbon Nanowires with Pseudocapacitive Properties as Advanced Materials for High‐Energy Lithium‐Ion Capacitors. Advanced Materials. https://doi.org/10.1002/adma.201700142
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