The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Delocalized Spin States in 2D Atomic Layers Realizing Enhanced Electrocatalytic Oxygen Evolution
Abstract
The electrocatalytic activity of transition‐metal‐based compounds is strongly related to the spin states of metal atoms. However, the ways for regulation of spin states of catalysts are still limited, and the underlying relationship between the spin states and catalytic activities remains unclear. Herein, for the first time, by taking Ni II‐based compounds without high or low spin states for example, it is shown that their spin states can be delocalized after introducing structural distortion to the atomic layers. The delocalized spin states for Ni atoms can provide not only high electrical conductivity but also low adsorption energy between the active sites and reaction intermediates for the system. As expected, the ultrathin nanosheets of nickel‐chalcogenides with structural distortions show dramatically enhanced activity in electrocatalytic oxygen evolution compared to their corresponding bulk samples. This work establishes new way for the design of advanced electrocatalysts in transition‐metal‐based compounds via regulation of spin states.
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Cites
Nanostructured Nickel Phosphide as an Electrocatalyst for the Hydrogen Evolution Reaction
Popczun, E. J., McKone, J. R., Read, C. G., Biacchi, A. J., Wiltrout, A. M., Lewis, N. S., & Schaak, R. E. (2013) · Journal of the American Chemical Society · doi:10.1021/ja403440e · Cited by 2,911
Enhanced catalytic activity in strained chemically exfoliated WS2 nanosheets for hydrogen evolution
Voiry, D., Yamaguchi, H., Li, J., Silva, R., Alves, D. C. B., Fujita, T., Chen, M., Asefa, T., Shenoy, V. B., Eda, G., et al. (2013) · Nature Materials · doi:10.1038/nmat3700 · Cited by 2,641
Metallic Nickel Nitride Nanosheets Realizing Enhanced Electrochemical Water Oxidation
Xu, K., Chen, P., Li, X., Tong, Y., Ding, H., Wu, X., Chu, W., Peng, Z., Wu, C., & Xie, Y. (2015) · Journal of the American Chemical Society · doi:10.1021/ja5119495 · Cited by 1,115
Self-citationLow Overpotential in Vacancy-Rich Ultrathin CoSe2 Nanosheets for Water Oxidation
Liu, Y., Cheng, H., Lyu, M., Fan, S., Liu, Q., Zhang, W., Zhi, Y., Wang, C., Xiao, C., Wei, S., et al. (2014) · Journal of the American Chemical Society · doi:10.1021/ja5085157 · Cited by 1,094
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Cited by
Manipulating spin polarization of titanium dioxide for efficient photocatalysis
Pan, L., Ai, M., Huang, C., Yin, L., Liu, X., Zhang, R., Wang, S., Jiang, Z., Zhang, X., Zou, J.-J., et al. (2020) · Nature Communications · doi:10.1038/s41467-020-14333-w · Cited by 543
Self-citationLi, C., Cao, Q., Wang, F., Xiao, Y., Li, Y., Delaunay, J.-J., & Zhu, H. (2018) · Chemical Society Reviews · doi:10.1039/c8cs00067k · Cited by 494
Metal Atom‐Doped Co 3 O 4 Hierarchical Nanoplates for Electrocatalytic Oxygen Evolution
Zhang, S. L., Guan, B. Y., Lu, X. F., Xi, S., Du, Y., & Lou, X. W. (. (2020) · Advanced Materials · doi:10.1002/adma.202002235 · Cited by 454
Porous Two-Dimensional Materials for Photocatalytic and Electrocatalytic Applications
Wang, H., Liu, X., Niu, P., Wang, S., Shi, J., & Li, L. (2020) · Matter · doi:10.1016/j.matt.2020.04.002 · Cited by 435
Self-citationFeS2/CoS2 Interface Nanosheets as Efficient Bifunctional Electrocatalyst for Overall Water Splitting
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Metadata
- Authors
- Chen, S., Kang, Z., Hu, X., Zhang, X., Wang, H., Xie, J., Zheng, X., Yan, W., Pan, B., & Xie, Y.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-06-08
- Volume
- 29
- Issue
- 30
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2623993588
- Cited by
- 187
- References
- 4
- FWCI
- 5.12
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, S., Kang, Z., Hu, X., Zhang, X., Wang, H., Xie, J., Zheng, X., Yan, W., Pan, B., & Xie, Y. (2017). Delocalized Spin States in 2D Atomic Layers Realizing Enhanced Electrocatalytic Oxygen Evolution. Advanced Materials. https://doi.org/10.1002/adma.201701687
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