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The Concept of “Noble, Heteroatom‐Doped Carbons,” Their Directed Synthesis by Electronic Band Control of Carbonization, and Applications in Catalysis and Energy Materials
Abstract
Carbonization of organic compounds with a highest occupied molecular orbital (HOMO) level more positive than 1.3 V practically automatically results in highly sp 2‐conjugated, heteroatom‐doped carbons. Due to the stability of the starting compounds, carbon bond formation is restricted to result in morphologies with a surprisingly high local order which as such are noble, i.e., they are hard to oxidize and combust. The work function of electrons in these systems is so positive that the systems usually accept electrons, i.e., they oxidize other matter rather than being oxidized. Such noble, heteroatom‐doped carbons have been proven to be efficient, metal‐free electrocatalysts, but can be also beneficially used in the manufacturing of carbon nanomaterials for energy applications or as highly active, non‐innocent catalytic supports.
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Cites
Efficient storage mechanisms for building better supercapacitors
Salanne, M., Rotenberg, B., Naoi, K., Kaneko, K., Taberna, P.-L., Grey, C. P., Dunn, B., & Simon, P. (2016) · Nature Energy · doi:10.1038/nenergy.2016.70 · Cited by 2,181
Engineering carbon materials from the hydrothermal carbonization process of biomass
Hu, B., Wang, K., Wu, L., Yu, S., Antonietti, M., & Titirici, M. (2010) · Advanced Materials · doi:10.1002/adma.200902812 · Cited by 1,765
Self-citationThe role of carbon materials in heterogeneous catalysis
Rodríguez-reinoso, F. (1998) · Carbon · doi:10.1016/s0008-6223(97)00173-5 · Cited by 1,760
Recent developments of carbon-based electrocatalysts for hydrogen evolution reaction
Zhou, W., Jia, J., Lu, J., Yang, L., Hou, D., Li, G., & Chen, S. (2016) · Nano Energy · doi:10.1016/j.nanoen.2016.08.027 · Cited by 744
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Control of metal-support interactions in heterogeneous catalysts to enhance activity and selectivity
van Deelen, T. W., Hernández Mejía, C., & de Jong, K. P. (2019) · Nature Catalysis · doi:10.1038/s41929-019-0364-x · Cited by 2,349
Comprehensive Understanding of the Thriving Ambient Electrochemical Nitrogen Reduction Reaction
Zhao, X., Hu, G., Chen, G., Zhang, H., Zhang, S., & Wang, H. (2021) · Advanced Materials · doi:10.1002/adma.202007650 · Cited by 503
Photoredox Catalytic Organic Transformations using Heterogeneous Carbon Nitrides
Savateev, A., Ghosh, I., König, B., & Antonietti, M. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201802472 · Cited by 477
Self-citationZhang, G., Li, G., Heil, T., Zafeiratos, S., Lai, F., Savateev, A., Antonietti, M., & Wang, X. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201811938 · Cited by 391
Self-citationQin, Q., Heil, T., Antonietti, M., & Oschatz, M. (2018) · Small Methods · doi:10.1002/smtd.201800202 · Cited by 257
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Metadata
- Authors
- Antonietti, M., & Oschatz, M.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2018-03-26
- Volume
- 30
- Issue
- 21
- Pages
- e1706836-e1706836
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2793402651
- Cited by
- 180
- References
- 4
- FWCI
- 5.66
- Type
- journal article
- Language
- en
- Open access
- closed
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