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The Rise of Hydrogen Peroxide as the Main Product by Metal‐Free Catalysis in Oxygen Reductions
Abstract
One of the recent trends in electrocatalytic reactions involves the oxygen reduction reaction (ORR), where a new paradigm has been shaped to exploit this reaction for the synthesis of hydrogen peroxide (H 2 O 2). H 2 O 2 is a very versatile chemical of high commercial value, prepared currently through poorly sustainable processes. The emergence of metal‐free carbon catalysts for the selective synthesis of H 2 O 2 is expected to revolutionize ORR research, beckoning at the development of new industrial schemes. The complexities of the mechanism and the factors dominating the selectivity of the process have been unveiled through a combination of theoretical and experimental studies.
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Citations
Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Cited by
Highly selective oxygen reduction to hydrogen peroxide on transition metal single atom coordination
Jiang, K., Back, S., Akey, A. J., Xia, C., Hu, Y., Liang, W., Schaak, D., Stavitski, E., Nørskov, J. K., Siahrostami, S., et al. (2019) · Nature Communications · doi:10.1038/s41467-019-11992-2 · Cited by 820
Gao, J., Yang, H. B., Huang, X., Hung, S.-F., Cai, W., Jia, C., Miao, S., Chen, H. M., Yang, X., Huang, Y., et al. (2020) · Chem · doi:10.1016/j.chempr.2019.12.008 · Cited by 734
Zeng, X., Liu, Y., Kang, Y., Li, Q., Xia, Y., Zhu, Y., Hou, H., Uddin, M. H., Gengenbach, T. R., Xia, D., et al. (2020) · ACS Catalysis · doi:10.1021/acscatal.9b05247 · Cited by 482
Zhao, Q., Wang, Y., Lai, W.-H., Xiao, F., Lyu, Y., Liao, C., & Shao, M. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00878a · Cited by 269
Bioinspired and Bioderived Aqueous Electrocatalysis
Barrio, J., Pedersen, A., Favero, S., Luo, H., Wang, M., Sarma, S. C., Feng, J., Ngoc, L. T. T., Kellner, S., Li, A. Y., et al. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00429 · Cited by 80
Metadata
- Authors
- Melchionna, M., Fornasiero, P., & Prato, M.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2018-08-17
- Volume
- 31
- Issue
- 13
- Pages
- e1802920-e1802920
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2885206286
- Cited by
- 380
- References
- 1
- FWCI
- 6.73
- Type
- journal article
- Language
- en
- Open access
- closed
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- Melchionna, M., Fornasiero, P., & Prato, M. (2019). The Rise of Hydrogen Peroxide as the Main Product by Metal‐Free Catalysis in Oxygen Reductions. Advanced Materials. https://doi.org/10.1002/adma.201802920
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