The DOI matches its Crossref record; 39 of the 39 references it cites were found in a registry or an index.
An Electron/Ion Dual‐Conductive Alloy Framework for High‐Rate and High‐Capacity Solid‐State Lithium‐Metal Batteries
Abstract
The solid‐state Li battery is a promising energy‐storage system that is both safe and features a high energy density. A main obstacle to its application is the poor interface contact between the solid electrodes and the ceramic electrolyte. Surface treatment methods have been proposed to improve the interface of the ceramic electrolytes, but they are generally limited to low‐capacity or short‐term cycling. Herein, an electron/ion dual‐conductive solid framework is proposed by partially dealloying the Li–Mg alloy anode on a garnet‐type solid‐state electrolyte. The Li–Mg alloy framework serves as a solid electron/ion dual‐conductive Li host during cell cycling, in which the Li metal can cycle as a Li‐rich or Li‐deficient alloy anode, free from interface deterioration or volume collapse. Thus, the capacity, current density, and cycle life of the solid Li anode are improved. The cycle capability of this solid anode is demonstrated by cycling for 500 h at 1 mA cm−2, followed by another 500 h at 2 mA cm−2 without short‐circuiting, realizing a record high cumulative capacity of 750 mA h cm−2 for garnet‐type all‐solid‐state Li batteries. This alloy framework with electron/ion dual‐conductive pathways creates the possibility to realize high‐energy solid‐state Li batteries with extended lifespans.
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Cites
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Cited by
Physicochemical Concepts of the Lithium Metal Anode in Solid-State Batteries
Krauskopf, T., Richter, F. H., Zeier, W. G., & Janek, J. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00431 · Cited by 892
Duan, H., Fan, M., Chen, W., Li, J., Wang, P., Wang, W., Shi, J., Yin, Y., Wan, L., & Guo, Y. (2019) · Advanced Materials · doi:10.1002/adma.201807789 · Cited by 466
Zheng, J., Kim, M. S., Tu, Z., Choudhury, S., Tang, T., & Archer, L. A. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00883g · Cited by 466
Krauskopf, T., Mogwitz, B., Rosenbach, C., Zeier, W. G., & Janek, J. (2019) · Advanced Energy Materials · doi:10.1002/aenm.201902568 · Cited by 438
Jiang, Z., Wang, S., Chen, X., Yang, W., Yao, X., Hu, X., Han, Q., & Wang, H. (2020) · Advanced Materials · doi:10.1002/adma.201906221 · Cited by 266
Metadata
- Authors
- Yang, C., Xie, H., Ping, W., Fu, K., Liu, B., Rao, J., Dai, J., Wang, C., Pastel, G., & Hu, L.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2018-11-21
- Volume
- 31
- Issue
- 3
- Pages
- e1804815-e1804815
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2900762588
- Cited by
- 317
- References
- 39
- FWCI
- 11.76
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yang, C., Xie, H., Ping, W., Fu, K., Liu, B., Rao, J., Dai, J., Wang, C., Pastel, G., & Hu, L. (2019). An Electron/Ion Dual‐Conductive Alloy Framework for High‐Rate and High‐Capacity Solid‐State Lithium‐Metal Batteries. Advanced Materials. https://doi.org/10.1002/adma.201804815
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