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High‐Entropy Oxides: Fundamental Aspects and Electrochemical Properties
Open accessAbstract
High‐entropy materials, especially high‐entropy alloys and oxides, have gained significant interest over the years due to their unique structural characteristics and correlated possibilities for tailoring of functional properties. The developments in the area of high‐entropy oxides are highlighted here, with emphasis placed on their fundamental understanding, including entropy‐dominated phase‐stabilization effects and prospective applications, e.g., in the field of electrochemical energy storage. Critical comments on the different classes of high‐entropy oxides are made and the underlying principles for the observed properties are summarized. The diversity of materials design, provided by the entropy‐mediated phase‐stabilization concept, allows engineering of new oxide candidates for practical applications, warranting further studies in this emerging field of materials science.
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Citations
Cited by
Oses, C., Toher, C., & Curtarolo, S. (2020) · Nature Reviews Materials · doi:10.1038/s41578-019-0170-8 · Cited by 2,081
Transition metal nitrides for electrochemical energy applications
Wang, H., Li, J., Li, K., Lin, Y., Chen, J., Gao, L., Nicolosi, V., Xiao, X., & Lee, J.-M. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00415d · Cited by 983
High-entropy energy materials: challenges and new opportunities
Ma, Y., Ma, Y., Wang, Q., Schweidler, S., Botros, M., Fu, T., Hahn, H., Brezesinski, T., & Breitung, B. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00505g · Cited by 963
Self-citationReview of high entropy ceramics: design, synthesis, structure and properties
Zhang, R.-Z., & Reece, M. J. (2019) · Journal of Materials Chemistry A · doi:10.1039/c9ta05698j · Cited by 760
High entropy spinel oxide nanoparticles for superior lithiation–delithiation performance
Nguyen, T. X., Patra, J., Chang, J.-K., & Ting, J.-M. (2020) · Journal of Materials Chemistry A · doi:10.1039/d0ta04844e · Cited by 341
Metadata
- Authors
- Sarkar, A., Wang, Q., Schiele, A., Chellali, M. R., Bhattacharya, S. S., Wang, D., Brezesinski, T., Hahn, H., Velasco, L., & Breitung, B.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2019-03-06
- Volume
- 31
- Issue
- 26
- Pages
- e1806236-e1806236
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2922252406
- Cited by
- 1,234
- References
- 0
- FWCI
- 43.96
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Sarkar, A., Wang, Q., Schiele, A., Chellali, M. R., Bhattacharya, S. S., Wang, D., Brezesinski, T., Hahn, H., Velasco, L., & Breitung, B. (2019). High‐Entropy Oxides: Fundamental Aspects and Electrochemical Properties. Advanced Materials. https://doi.org/10.1002/adma.201806236
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