The DOI matches its Crossref record; 68 of the 68 references it cites were found in a registry or an index.
Ambient Fast Synthesis and Active Sites Deciphering of Hierarchical Foam‐Like Trimetal–Organic Framework Nanostructures as a Platform for Highly Efficient Oxygen Evolution Electrocatalysis
Abstract
Metal–organic frameworks (MOFs) have attracted tremendous interest due to their promising applications including electrocatalysis originating from their unique structural features. However, it remains a challenge to directly use MOFs for oxygen electrocatalysis because it is quite difficult to manipulate their dimension, composition, and morphology of the MOFs with abundant active sites. Here, a facile ambient temperature synthesis of unique NiCoFe‐based trimetallic MOF nanostructures with foam‐like architecture is reported, which exhibit extraordinary oxygen evolution reaction (OER) activity as directly used catalyst in alkaline condition. Specifically, the (Ni 2 Co 1)0.925 Fe 0.075‐MOF‐NF delivers a minimum overpotential of 257 mV to reach the current density of 10 mA cm−2 with a small Tafel slope of 41.3 mV dec−1 and exhibits high durability after long‐term testing. More importantly, the deciphering of the possible origination of the high activity is performed through the characterization of the intermediates during the OER process, where the electrochemically transformed metal hydroxides and oxyhydroxides are confirmed as the active species.
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Cites
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Cited by
Non-noble metal-nitride based electrocatalysts for high-performance alkaline seawater electrolysis
Yu, L., Zhu, Q., Song, S., McElhenny, B., Wang, D., Wu, C., Qin, Z., Bao, J., Yu, Y., Chen, S., et al. (2019) · Nature Communications · doi:10.1038/s41467-019-13092-7 · Cited by 1,333
Self-citationYu, M., Budiyanto, E., & Tüysüz, H. (2022) · Angewandte Chemie International Edition · doi:10.1002/anie.202103824 · Cited by 771
Metal–organic frameworks and their derivatives as electrocatalysts for the oxygen evolution reaction
Du, J., Li, F., & Sun, L. (2021) · Chemical Society Reviews · doi:10.1039/d0cs01191f · Cited by 578
Liu, X., Meng, J., Zhu, J., Huang, M., Wen, B., Guo, R., & Mai, L. (2021) · Advanced Materials · doi:10.1002/adma.202007344 · Cited by 438
Recent Advancements in Electrochemical Hydrogen Production via Hybrid Water Splitting
Qian, Q., Zhu, Y., Ahmad, N., Feng, Y., Zhang, H., Cheng, M., Liu, H., Xiao, C., Zhang, G., & Xie, Y. (2024) · Advanced Materials · doi:10.1002/adma.202306108 · Cited by 399
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Metadata
- Authors
- Qian, Q., Li, Y., Liu, Y., Yu, L., & Zhang, G.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2019-04-11
- Volume
- 31
- Issue
- 23
- Pages
- e1901139-e1901139
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2936440807
- Cited by
- 517
- References
- 68
- FWCI
- 15.31
- Type
- journal article
- Language
- en
- Open access
- closed
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- Qian, Q., Li, Y., Liu, Y., Yu, L., & Zhang, G. (2019). Ambient Fast Synthesis and Active Sites Deciphering of Hierarchical Foam‐Like Trimetal–Organic Framework Nanostructures as a Platform for Highly Efficient Oxygen Evolution Electrocatalysis. Advanced Materials. https://doi.org/10.1002/adma.201901139
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