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Side Chain Redistribution as a Strategy to Boost Organic Electrochemical Transistor Performance and Stability
Open accessAbstract
A series of glycolated polythiophenes for use in organic electrochemical transistors (OECTs) is designed and synthesized, differing in the distribution of their ethylene glycol chains that are tethered to the conjugated backbone. While side chain redistribution does not have a significant impact on the optoelectronic properties of the polymers, this molecular engineering strategy strongly impacts the water uptake achieved in the polymers. By careful optimization of the water uptake in the polymer films, OECTs with unprecedented steady‐state performances in terms of [μC*] and current retentions up to 98% over 700 electrochemical switching cycles are developed.
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Cited by
Vertical organic electrochemical transistors for complementary circuits
Huang, W., Chen, J., Yao, Y., Zheng, D., Ji, X., Feng, L.-W., Moore, D., Glavin, N. R., Xie, M., Chen, Y., et al. (2023) · Nature · doi:10.1038/s41586-022-05592-2 · Cited by 423
Yang, K., Chen, Z., Wang, Y., & Guo, X. (2023) · Accounts of Materials Research · doi:10.1021/accountsmr.2c00237 · Cited by 72
Metadata
- Authors
- Moser, M., Hidalgo, T. C., Surgailis, J., Gladisch, J., Ghosh, S., Sheelamanthula, R., Thiburce, Q., Giovannitti, A., Salleo, A., Gasparini, N., Wadsworth, A., Zozoulenko, I., Berggren, M., Stavrinidou, E., Inal, S., & McCulloch, I.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2020-08-05
- Volume
- 32
- Issue
- 37
- Pages
- e2002748-e2002748
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W3047226408
- Cited by
- 329
- References
- 0
- FWCI
- 15.89
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- CoChat. (2026). Citation check: Side Chain Redistribution as a Strategy to Boost Organic Electrochemical Transistor Performance and Stability. https://app.cochat.ai/papers/10.1002/adma.202002748
- The paper
- Moser, M., Hidalgo, T. C., Surgailis, J., Gladisch, J., Ghosh, S., Sheelamanthula, R., Thiburce, Q., Giovannitti, A., Salleo, A., Gasparini, N., Wadsworth, A., Zozoulenko, I., Berggren, M., Stavrinidou, E., Inal, S., & McCulloch, I. (2020). Side Chain Redistribution as a Strategy to Boost Organic Electrochemical Transistor Performance and Stability. Advanced Materials. https://doi.org/10.1002/adma.202002748
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
