The DOI matches its Crossref record; 37 of the 37 references it cites were found in a registry or an index.
A MOF‐Derivative Decorated Hierarchical Porous Host Enabling Ultrahigh Rates and Superior Long‐Term Cycling of Dendrite‐Free Zn Metal Anodes
Abstract
Aqueous Zn metal batteries have attracted much attention due to their high intrinsic capacity, high safety, and low cost. Nevertheless, uncontrollable dendrite growth and adverse side reactions of Zn anodes seriously hinder their further application. Herein, a three‐dimensional (3D) porous graphene‐carbon nanotubes scaffold decorated with metal–organic framework derived ZnO/C nanoparticles (3D‐ZGC) is fabricated as the host for dendrite‐free Zn‐metal composite anodes. The zincophilic ZnO/C nanoparticles act as preferred deposition sites with low nucleation barriers to induce homogeneous Zn deposition. The mechanically robust 3D scaffold with high conductivity not only suppresses the formation of dendritic Zn by reducing the local current density and homogenizing Zn 2+ ion flux, but also inhibits volume changes during the long‐term plating/stripping process. As a result, the 3D‐ZGC composite anodes afford unprecedented Zn plating‐stripping stability at an ultrahigh current density of 20 mA cm‐2 for 1500 cycles with low overpotential (<65 mV) when used in a symmetric cell. When coupled with MnO 2 cathodes, the assembled Zn@3D‐ZGC//MnO 2 full batteries deliver an enhanced cycling stability for up to 6000 cycles at 2000 mA g‐1, demonstrating the potential of the 3D‐ZGC composite anode for advanced Zn metal batteries.
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Cites
“Water-in-salt” electrolyte enables high-voltage aqueous lithium-ion chemistries
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Highly reversible zinc metal anode for aqueous batteries
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Reversible aqueous zinc/manganese oxide energy storage from conversion reactions
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Scientific Challenges for the Implementation of Zn-Ion Batteries
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Fluorinated interphase enables reversible aqueous zinc battery chemistries
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Dendrites in Zn‐Based Batteries
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Surface‐Preferred Crystal Plane for a Stable and Reversible Zinc Anode
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Cited by
Recent Progress on Zn Anodes for Advanced Aqueous Zinc‐Ion Batteries
Nie, C., Wang, G., Wang, D., Wang, M., Gao, X., Bai, Z., Wang, N., Yang, J., Xing, Z., & Dou, S. (2023) · Advanced Energy Materials · doi:10.1002/aenm.202300606 · Cited by 561
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Metadata
- Authors
- Xue, P., Guo, C., Li, L., Li, H., Luo, D., Tan, L., & Chen, Z.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2022-02-26
- Volume
- 34
- Issue
- 14
- Pages
- e2110047-e2110047
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W4210323328
- Cited by
- 259
- References
- 37
- FWCI
- 15.66
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xue, P., Guo, C., Li, L., Li, H., Luo, D., Tan, L., & Chen, Z. (2022). A MOF‐Derivative Decorated Hierarchical Porous Host Enabling Ultrahigh Rates and Superior Long‐Term Cycling of Dendrite‐Free Zn Metal Anodes. Advanced Materials. https://doi.org/10.1002/adma.202110047
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