The DOI matches its Crossref record; 53 of the 53 references it cites were found in a registry or an index.
Zinc Single‐Atom‐Regulated Hard Carbons for High‐Rate and Low‐Temperature Sodium‐Ion Batteries
Abstract
Hard carbons, as one of the most commercializable anode materials for sodium‐ion batteries (SIBs), have to deal with the trade‐off between the rate capability and specific capacity or initial Columbic efficiency (ICE), and the fast performance decline at low temperature (LT) remains poorly understood. Here, a comprehensive regulation on the interfacial/bulk electrochemistry of hard carbons through atomic Zn doping is reported, which demonstrates a record‐high reversible capacity (546 mAh g−1), decent ICE (84%), remarkable rate capability (140 mAh g−1 @ 50 A g−1), and excellent LT capacity (443 mAh g−1 @ −40 °C), outperforming the state‐of‐the‐art literature. This work reveals that the Zn doping can generally induce a local electric field to enable fast bulk Na+ transportation, and meanwhile catalyze the decomposition of NaPF 6 to form a robust inorganic‐rich solid‐electrolyte interphase, which elaborates the underlying origin of the boosted electrochemical performance. Importantly, distinguished from room temperature, the intrinsic Na+ migration/desolvation ability of the electrolyte is disclosed to be the crucial rate‐determining factors for the SIB performance at LT. This work provides a fundamental understanding on the charge‐storage kinetics at varied temperatures.
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Citations
Cites
Expanded graphite as superior anode for sodium-ion batteries
Wen, Y., He, K., Zhu, Y., Han, F., Xu, Y., Matsuda, I., Ishii, Y., Cumings, J., & Wang, C. (2014) · Nature Communications · doi:10.1038/ncomms5033 · Cited by 1,894
Du, Z., Chen, X., Hu, W., Chuang, C., Xie, S., Hu, A., Yan, W., Kong, X., Wu, X., Ji, H., et al. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.8b12973 · Cited by 1,490
Electrolyte design for Li-ion batteries under extreme operating conditions
Xu, J., Zhang, J., Pollard, T. P., Li, Q., Tan, S., Hou, S., Wan, H., Chen, F., He, H., Hu, E., et al. (2023) · Nature · doi:10.1038/s41586-022-05627-8 · Cited by 970
Tailoring electrolyte solvation for Li metal batteries cycled at ultra-low temperature
Holoubek, J., Liu, H., Wu, Z., Yin, Y., Xing, X., Cai, G., Yu, S., Zhou, H., Pascal, T. A., Chen, Z., et al. (2021) · Nature Energy · doi:10.1038/s41560-021-00783-z · Cited by 851
An Isolated Zinc–Cobalt Atomic Pair for Highly Active and Durable Oxygen Reduction
Lu, Z., Wang, B., Hu, Y., Liu, W., Zhao, Y., Yang, R., Li, Z., Luo, J., Chi, B., Jiang, Z., et al. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201810175 · Cited by 675
Self-citationEmerging Era of Electrolyte Solvation Structure and Interfacial Model in Batteries
Cheng, H., Sun, Q., Li, L., Zou, Y., Wang, Y., Cai, T., Zhao, F., Liu, G., Ma, Z., Wahyudi, W., et al. (2022) · ACS Energy Letters · doi:10.1021/acsenergylett.1c02425 · Cited by 640
MgO‐Template Synthesis of Extremely High Capacity Hard Carbon for Na‐Ion Battery
Kamiyama, A., Kubota, K., Igarashi, D., Youn, Y., Tateyama, Y., Ando, H., Gotoh, K., & Komaba, S. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202013951 · Cited by 586
Huang, S., Li, Z., Wang, B., Zhang, J., Peng, Z., Qi, R., Wang, J., & Zhao, Y. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201706294 · Cited by 585
Self-citationLi, J., Zhang, H., Samarakoon, W., Shan, W., Cullen, D. A., Karakalos, S., Chen, M., Gu, D., More, K. L., Wang, G., et al. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201909312 · Cited by 558
Toward Critical Electrode/Electrolyte Interfaces in Rechargeable Batteries
Yan, C., Xu, R., Xiao, Y., Ding, J., Xu, L., Li, B., & Huang, J. (2020) · Advanced Functional Materials · doi:10.1002/adfm.201909887 · Cited by 510
Cited by
Emerging Chemistry for Wide-Temperature Sodium-Ion Batteries
Zhang, F., He, B., Xin, Y., Zhu, T., Zhang, Y., Wang, S., Li, W., Yang, Y., & Tian, H. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.3c00728 · Cited by 357
Metadata
- Authors
- Lu, Z., Wang, J., Feng, W., Yin, X., Feng, X., Zhao, S., Li, C., Wang, R., Huang, Q., & Zhao, Y.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2023-05-07
- Volume
- 35
- Issue
- 26
- Pages
- e2211461-e2211461
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W4353017626
- Cited by
- 373
- References
- 53
- FWCI
- 27.34
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lu, Z., Wang, J., Feng, W., Yin, X., Feng, X., Zhao, S., Li, C., Wang, R., Huang, Q., & Zhao, Y. (2023). Zinc Single‐Atom‐Regulated Hard Carbons for High‐Rate and Low‐Temperature Sodium‐Ion Batteries. Advanced Materials. https://doi.org/10.1002/adma.202211461
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