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Cited by 146Aerogels and thermal insulationMesoporous Materials and CatalysisAdvanced ceramic materials synthesis

Mechanically Strengthened Aerogels through Multiscale, Multicompositional, and Multidimensional Approaches: A Review

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Parale, Vinayak G., Kim, Taehee, Choi, Haryeong, Phadtare, Varsha D., Dhavale, Rushikesh P., Kanamori, Kazuyoshi, Park, Hyung‐Ho·2024·Advanced Materials
DOI 10.1002/adma.202307772
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Abstract

In recent decades, aerogels have attracted tremendous attention in academia and industry as a class of lightweight and porous multifunctional nanomaterial. Despite their wide application range, the low mechanical durability hinders their processing and handling, particularly in applications requiring complex physical structures. "Mechanically strengthened aerogels" have emerged as a potential solution to address this drawback. Since the first report on aerogels in 1931, various modified synthesis processes have been introduced in the last few decades to enhance the aerogel mechanical strength, further advancing their multifunctional scope. This review summarizes the state-of-the-art developments of mechanically strengthened aerogels through multicompositional and multidimensional approaches. Furthermore, new trends and future directions for as prevailed commercialization of aerogels as plastic materials are discussed.

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  • Freeze-drying has disadvantages including difficulty in creating monoliths and the requirement to switch out solvents while avoiding production of pores with a micrometer size of 10 μm.

    “Some disadvantages of this approach include the difficulty in creating monoliths and the requirement to switch out solvents while avoiding the production of pores with a micrometer size of 10 μm.”

    From Silica Aerogels as a Promising Vehicle for Effective Water Splitting for Hydrogen Production (2025) · cites this paper as [2]

    The “Freeze drying process” section identifies difficulty making monoliths and the need to exchange solvents while preventing micron-size pores as drawbacks of freeze-drying. It specifies pores with diameters **more than 10 μm**, whereas the citing sentence describes pores of 10 μm. (LLM, conf=0.85)

    Experimental — accuracy not yet measured

  • The pore diameter and shape of an aerogel can be altered at the nano level to achieve versatile properties such as high surface area, low density, large pore size, and low thermal conductivity.

    “The pore diameter and the shape of the aerogel can be altered at the nano level to achieve versatile properties, like a high surface area, low density, a large pore size, and low thermal conductivity [2].”

    From Silica Aerogels as a Promising Vehicle for Effective Water Splitting for Hydrogen Production (2025) · cites this paper as [2]

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Authors
Parale, V. G., Kim, T., Choi, H., Phadtare, V. D., Dhavale, R. P., Kanamori, K., & Park, H.
Affiliations
  • Yonsei University (KR)
  • Kyoto University (JP)
Corresponding author
  • Kanamori, Kazuyoshi
  • Park, Hyung‐Ho
ORCID
Venue
Advanced Materials
Publisher
Wiley
Published
2024-02-04
Volume
36
Issue
18
Pages
e2307772-e2307772
ISSN
  • 0935-9648 (ISSN-L)
  • 1521-4095
DOI
10.1002/adma.202307772
OpenAlex
W4388213683
Cited by
146
References
561
Citations by year
2026: 32 · 2025: 88 · 2024: 26
FWCI
4.41
Type
journal article
Language
en
Open access
Licence
Locations
  • Advanced Materials (publishedVersion, cc-by)
  • PubMed (publishedVersion)
  • Institutional Repositories DataBase (IRDB) (submittedVersion, cc-by)
  • Kyoto University Research Information Repository (Kyoto University) (submittedVersion, cc-by)
Funders
National Research Foundation of Korea (2020R1A5A1019131)
Topics
  • Physical Sciences › Chemistry › Spectroscopy › Aerogels and thermal insulation
  • Physical Sciences › Materials Science › Materials Chemistry › Mesoporous Materials and Catalysis
  • Physical Sciences › Materials Science › Ceramics and Composites › Advanced ceramic materials synthesis
Keywords
aerogels, mechanical strength, mechanical durability, multiscale composites, nanoporous materials, plastics

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